Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions

Research output: Contribution to journalArticleResearchpeer review

Authors

  • J Thielking
  • K Zhang
  • J Tiedau
  • J Zander
  • G Zitzer
  • M v Okhapkin
  • Ekkehard Peik

External Research Organisations

  • Physikalisch-Technische Bundesanstalt PTB
View graph of relations

Details

Original languageEnglish
Article number083026
Pages (from-to)083026
JournalNew journal of physics
Volume25
Issue number8
Publication statusPublished - 14 Aug 2023
Externally publishedYes

Abstract

A tunable vacuum-ultraviolet (VUV) laser source based on four-wave frequency mixing in xenon is presented. Using seed radiation from two continuous-wave lasers, the system allows for precise control of the VUV frequency and is developed for the resonant laser excitation of the Th-229 nucleus to its low-energy isomeric state. The system is prepared to operate in a wide scanning range from 148 nm to 155 nm. The source produces pulses of 6-10 ns duration with up to 40 µJ energy and is coupled via a vacuum beamline to a linear radiofrequency ion trap. In a first implementation of VUV laser spectroscopy of trapped Th + ions we excite three previously unknown resonance lines near 149 nm wavelength to electronic levels that are close to the Th-229 isomer energy. The resonances are detected and analyzed via fluorescence of the excited Th + ions. An analysis of the lineshape is used to estimate the linewidth of the VUV radiation to be in the range of ⩽ 6 GHz, dominated by phase noise that is enhanced in harmonic generation and in the four-wave mixing process. The prospects for the use of the system in nuclear laser spectroscopy of Th-229 are discussed.

Keywords

    nuclear laser excitation, trapped ions, VUV laser

ASJC Scopus subject areas

Cite this

Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions. / Thielking, J; Zhang, K; Tiedau, J et al.
In: New journal of physics, Vol. 25, No. 8, 083026, 14.08.2023, p. 083026.

Research output: Contribution to journalArticleResearchpeer review

Thielking, J, Zhang, K, Tiedau, J, Zander, J, Zitzer, G, Okhapkin, MV & Peik, E 2023, 'Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions', New journal of physics, vol. 25, no. 8, 083026, pp. 083026. https://doi.org/10.1088/1367-2630/aced1b
Thielking, J., Zhang, K., Tiedau, J., Zander, J., Zitzer, G., Okhapkin, M. V., & Peik, E. (2023). Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions. New journal of physics, 25(8), 083026. Article 083026. https://doi.org/10.1088/1367-2630/aced1b
Thielking J, Zhang K, Tiedau J, Zander J, Zitzer G, Okhapkin MV et al. Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions. New journal of physics. 2023 Aug 14;25(8):083026. 083026. doi: 10.1088/1367-2630/aced1b
Thielking, J ; Zhang, K ; Tiedau, J et al. / Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions. In: New journal of physics. 2023 ; Vol. 25, No. 8. pp. 083026.
Download
@article{5ba3fcb05705488b9a9cd10c6beef399,
title = "Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions",
abstract = "A tunable vacuum-ultraviolet (VUV) laser source based on four-wave frequency mixing in xenon is presented. Using seed radiation from two continuous-wave lasers, the system allows for precise control of the VUV frequency and is developed for the resonant laser excitation of the Th-229 nucleus to its low-energy isomeric state. The system is prepared to operate in a wide scanning range from 148 nm to 155 nm. The source produces pulses of 6-10 ns duration with up to 40 µJ energy and is coupled via a vacuum beamline to a linear radiofrequency ion trap. In a first implementation of VUV laser spectroscopy of trapped Th + ions we excite three previously unknown resonance lines near 149 nm wavelength to electronic levels that are close to the Th-229 isomer energy. The resonances are detected and analyzed via fluorescence of the excited Th + ions. An analysis of the lineshape is used to estimate the linewidth of the VUV radiation to be in the range of ⩽ 6 GHz, dominated by phase noise that is enhanced in harmonic generation and in the four-wave mixing process. The prospects for the use of the system in nuclear laser spectroscopy of Th-229 are discussed.",
keywords = "nuclear laser excitation, trapped ions, VUV laser",
author = "J Thielking and K Zhang and J Tiedau and J Zander and G Zitzer and Okhapkin, {M v} and Ekkehard Peik",
note = "Publisher Copyright: {\textcopyright} 2023 The Author(s). Published by IOP Publishing Ltd on behalf of the Institute of Physics and Deutsche Physikalische Gesellschaft.",
year = "2023",
month = aug,
day = "14",
doi = "10.1088/1367-2630/aced1b",
language = "English",
volume = "25",
pages = "083026",
journal = "New journal of physics",
issn = "1367-2630",
publisher = "IOP Publishing Ltd.",
number = "8",

}

Download

TY - JOUR

T1 - Vacuum-ultraviolet laser source for spectroscopy of trapped thorium ions

AU - Thielking, J

AU - Zhang, K

AU - Tiedau, J

AU - Zander, J

AU - Zitzer, G

AU - Okhapkin, M v

AU - Peik, Ekkehard

N1 - Publisher Copyright: © 2023 The Author(s). Published by IOP Publishing Ltd on behalf of the Institute of Physics and Deutsche Physikalische Gesellschaft.

PY - 2023/8/14

Y1 - 2023/8/14

N2 - A tunable vacuum-ultraviolet (VUV) laser source based on four-wave frequency mixing in xenon is presented. Using seed radiation from two continuous-wave lasers, the system allows for precise control of the VUV frequency and is developed for the resonant laser excitation of the Th-229 nucleus to its low-energy isomeric state. The system is prepared to operate in a wide scanning range from 148 nm to 155 nm. The source produces pulses of 6-10 ns duration with up to 40 µJ energy and is coupled via a vacuum beamline to a linear radiofrequency ion trap. In a first implementation of VUV laser spectroscopy of trapped Th + ions we excite three previously unknown resonance lines near 149 nm wavelength to electronic levels that are close to the Th-229 isomer energy. The resonances are detected and analyzed via fluorescence of the excited Th + ions. An analysis of the lineshape is used to estimate the linewidth of the VUV radiation to be in the range of ⩽ 6 GHz, dominated by phase noise that is enhanced in harmonic generation and in the four-wave mixing process. The prospects for the use of the system in nuclear laser spectroscopy of Th-229 are discussed.

AB - A tunable vacuum-ultraviolet (VUV) laser source based on four-wave frequency mixing in xenon is presented. Using seed radiation from two continuous-wave lasers, the system allows for precise control of the VUV frequency and is developed for the resonant laser excitation of the Th-229 nucleus to its low-energy isomeric state. The system is prepared to operate in a wide scanning range from 148 nm to 155 nm. The source produces pulses of 6-10 ns duration with up to 40 µJ energy and is coupled via a vacuum beamline to a linear radiofrequency ion trap. In a first implementation of VUV laser spectroscopy of trapped Th + ions we excite three previously unknown resonance lines near 149 nm wavelength to electronic levels that are close to the Th-229 isomer energy. The resonances are detected and analyzed via fluorescence of the excited Th + ions. An analysis of the lineshape is used to estimate the linewidth of the VUV radiation to be in the range of ⩽ 6 GHz, dominated by phase noise that is enhanced in harmonic generation and in the four-wave mixing process. The prospects for the use of the system in nuclear laser spectroscopy of Th-229 are discussed.

KW - nuclear laser excitation

KW - trapped ions

KW - VUV laser

UR - http://www.scopus.com/inward/record.url?scp=85168559072&partnerID=8YFLogxK

U2 - 10.1088/1367-2630/aced1b

DO - 10.1088/1367-2630/aced1b

M3 - Article

VL - 25

SP - 083026

JO - New journal of physics

JF - New journal of physics

SN - 1367-2630

IS - 8

M1 - 083026

ER -