Details
| Original language | English |
|---|---|
| Pages (from-to) | 21459-21468 |
| Number of pages | 10 |
| Journal | ACS Omega |
| Volume | 4 |
| Issue number | 25 |
| Early online date | 5 Dec 2019 |
| Publication status | Published - 17 Dec 2019 |
| Externally published | Yes |
Abstract
Optically assisted electrical generation of umbilic defects, arising in homeotropically aligned nematic liquid crystal cells and known as topological templates for the generation of optical vortices, are reported in nematic liquid crystals with positive dielectric anisotropy in detail. It is shown that nematic liquid crystals with positive dielectric anisotropy can serve as a stable and efficient medium for the optical vortex generation from both linearly and circularly polarized input Gaussian beams. Hybrid cells made from a thin layer of nematic liquid crystal confined between a photoresponsive slab of iron-doped lithium niobate and a glass plate coated with an active material, i.e., indium tin oxide, were studied. Exposure to a laser beam locally induces a photovoltaic field in the iron-doped lithium niobate substrate, which can penetrate into the liquid crystal film and induce realignment of molecules. The photovoltaic field drives charge carrier accumulation at the interface of indium tin oxide with the liquid crystal, which effectively modifies the shape and symmetry of the electric field. The photovoltaic field has a continuous radial distribution in the transverse xy-plane, weakening with increasing distance from the light irradiation center, where the electric field is normal to the cell plane. Umbilics are created as a result of the liquid crystal tendency to realign parallel to the electric field. Numerical studies of the transmitted intensity profiles in between linear polarizers reveal optical vortex pattern (of four and eight brushes) characteristics for the umbilical defects. The application of crossed circular polarizers results in annular-shaped intensity patterns as a result of spin-to-orbital angular momentum conversions, which give rise to the optical vortices.
ASJC Scopus subject areas
- Chemistry(all)
- General Chemistry
- Chemical Engineering(all)
- General Chemical Engineering
Sustainable Development Goals
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In: ACS Omega, Vol. 4, No. 25, 17.12.2019, p. 21459-21468.
Research output: Contribution to journal › Article › Research › peer review
}
TY - JOUR
T1 - Theoretical Prediction of Umbilics Creation in Nematic Liquid Crystals with Positive Dielectric Anisotropy
AU - Habibpourmoghadam, Atefeh
N1 - Funding Information: The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acsomega.9b03158 . Discussion on the charge carrier accumulation in the ITO thin film; photovoltaic electric field responsible for the charge accumilation; numerically obtained electric potential distribution; charge carrier density ( PDF ) The research work was partially funded by the US Air Force Office of Scientific Research (AFOSR) through the European Office of Aerospace Research & Development (EOARD) Grant FA9550-18-1-7002 and partially by the German Research Council (DFG) Grant LO 1922/4-1, which are gracefully acknowledged. The author declares no competing financial interest.
PY - 2019/12/17
Y1 - 2019/12/17
N2 - Optically assisted electrical generation of umbilic defects, arising in homeotropically aligned nematic liquid crystal cells and known as topological templates for the generation of optical vortices, are reported in nematic liquid crystals with positive dielectric anisotropy in detail. It is shown that nematic liquid crystals with positive dielectric anisotropy can serve as a stable and efficient medium for the optical vortex generation from both linearly and circularly polarized input Gaussian beams. Hybrid cells made from a thin layer of nematic liquid crystal confined between a photoresponsive slab of iron-doped lithium niobate and a glass plate coated with an active material, i.e., indium tin oxide, were studied. Exposure to a laser beam locally induces a photovoltaic field in the iron-doped lithium niobate substrate, which can penetrate into the liquid crystal film and induce realignment of molecules. The photovoltaic field drives charge carrier accumulation at the interface of indium tin oxide with the liquid crystal, which effectively modifies the shape and symmetry of the electric field. The photovoltaic field has a continuous radial distribution in the transverse xy-plane, weakening with increasing distance from the light irradiation center, where the electric field is normal to the cell plane. Umbilics are created as a result of the liquid crystal tendency to realign parallel to the electric field. Numerical studies of the transmitted intensity profiles in between linear polarizers reveal optical vortex pattern (of four and eight brushes) characteristics for the umbilical defects. The application of crossed circular polarizers results in annular-shaped intensity patterns as a result of spin-to-orbital angular momentum conversions, which give rise to the optical vortices.
AB - Optically assisted electrical generation of umbilic defects, arising in homeotropically aligned nematic liquid crystal cells and known as topological templates for the generation of optical vortices, are reported in nematic liquid crystals with positive dielectric anisotropy in detail. It is shown that nematic liquid crystals with positive dielectric anisotropy can serve as a stable and efficient medium for the optical vortex generation from both linearly and circularly polarized input Gaussian beams. Hybrid cells made from a thin layer of nematic liquid crystal confined between a photoresponsive slab of iron-doped lithium niobate and a glass plate coated with an active material, i.e., indium tin oxide, were studied. Exposure to a laser beam locally induces a photovoltaic field in the iron-doped lithium niobate substrate, which can penetrate into the liquid crystal film and induce realignment of molecules. The photovoltaic field drives charge carrier accumulation at the interface of indium tin oxide with the liquid crystal, which effectively modifies the shape and symmetry of the electric field. The photovoltaic field has a continuous radial distribution in the transverse xy-plane, weakening with increasing distance from the light irradiation center, where the electric field is normal to the cell plane. Umbilics are created as a result of the liquid crystal tendency to realign parallel to the electric field. Numerical studies of the transmitted intensity profiles in between linear polarizers reveal optical vortex pattern (of four and eight brushes) characteristics for the umbilical defects. The application of crossed circular polarizers results in annular-shaped intensity patterns as a result of spin-to-orbital angular momentum conversions, which give rise to the optical vortices.
UR - http://www.scopus.com/inward/record.url?scp=85076246081&partnerID=8YFLogxK
UR - https://pubs.acs.org/page/policy/authorchoice_termsofuse.html
U2 - 10.1021/acsomega.9b03158
DO - 10.1021/acsomega.9b03158
M3 - Article
AN - SCOPUS:85076246081
VL - 4
SP - 21459
EP - 21468
JO - ACS Omega
JF - ACS Omega
IS - 25
ER -