The concept of laser-based conversion electron Mössbauer spectroscopy for a precise energy determination of 229m Th

Research output: Contribution to journalArticleResearchpeer review

Authors

  • Lars C. von der Wense
  • Benedict Seiferle
  • Christian Schneider
  • Justin Jeet
  • Ines Amersdorffer
  • Nicolas Arlt
  • Florian Zacherl
  • Raphael Haas
  • Dennis Renisch
  • Patrick Mosel
  • Philip Mosel
  • Milutin Kovacev
  • Uwe Morgner
  • Christoph E. Düllmann
  • Eric R. Hudson
  • Peter G. Thirolf

External Research Organisations

  • Ludwig-Maximilians-Universität München (LMU)
  • University of California (UCLA)
  • Johannes Gutenberg University Mainz
  • Helmholtz-Institut Mainz
  • GSI Helmholtz Centre for Heavy Ion Research
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Details

Original languageEnglish
Article number23
JournalHyperfine Interactions
Volume240
Issue number1
Publication statusE-pub ahead of print - 13 Mar 2019

Abstract

229 Th is the only nucleus currently under investigation for the development of a nuclear optical clock (NOC) of ultra-high accuracy. The insufficient knowledge of the first nuclear excitation energy of 229 Th has so far hindered direct nuclear laser spectroscopy of thorium ions and thus the development of a NOC. Here, a nuclear laser excitation scheme is detailed, which makes use of thorium atoms instead of ions. This concept, besides potentially leading to the first nuclear laser spectroscopy, would determine the isomeric energy to 40 μeV resolution, corresponding to 10 GHz, which is a 10 4 times improvement compared to the current best energy constraint. This would determine the nuclear isomeric energy to a sufficient accuracy to allow for nuclear laser spectroscopy of individual thorium ions in a Paul trap and thus the development of a single-ion nuclear optical clock.

Keywords

    Nuclear laser spectroscopy, Nuclear optical clock, Thorium-229

ASJC Scopus subject areas

Cite this

The concept of laser-based conversion electron Mössbauer spectroscopy for a precise energy determination of 229m Th. / von der Wense, Lars C.; Seiferle, Benedict; Schneider, Christian et al.
In: Hyperfine Interactions, Vol. 240, No. 1, 23, 13.03.2019.

Research output: Contribution to journalArticleResearchpeer review

von der Wense, LC, Seiferle, B, Schneider, C, Jeet, J, Amersdorffer, I, Arlt, N, Zacherl, F, Haas, R, Renisch, D, Mosel, P, Mosel, P, Kovacev, M, Morgner, U, Düllmann, CE, Hudson, ER & Thirolf, PG 2019, 'The concept of laser-based conversion electron Mössbauer spectroscopy for a precise energy determination of 229m Th', Hyperfine Interactions, vol. 240, no. 1, 23. https://doi.org/10.1007/s10751-019-1564-0, https://doi.org/10.48550/arXiv.1904.01245
von der Wense, L. C., Seiferle, B., Schneider, C., Jeet, J., Amersdorffer, I., Arlt, N., Zacherl, F., Haas, R., Renisch, D., Mosel, P., Mosel, P., Kovacev, M., Morgner, U., Düllmann, C. E., Hudson, E. R., & Thirolf, P. G. (2019). The concept of laser-based conversion electron Mössbauer spectroscopy for a precise energy determination of 229m Th. Hyperfine Interactions, 240(1), Article 23. Advance online publication. https://doi.org/10.1007/s10751-019-1564-0, https://doi.org/10.48550/arXiv.1904.01245
von der Wense LC, Seiferle B, Schneider C, Jeet J, Amersdorffer I, Arlt N et al. The concept of laser-based conversion electron Mössbauer spectroscopy for a precise energy determination of 229m Th. Hyperfine Interactions. 2019 Mar 13;240(1):23. Epub 2019 Mar 13. doi: 10.1007/s10751-019-1564-0, 10.48550/arXiv.1904.01245
von der Wense, Lars C. ; Seiferle, Benedict ; Schneider, Christian et al. / The concept of laser-based conversion electron Mössbauer spectroscopy for a precise energy determination of 229m Th. In: Hyperfine Interactions. 2019 ; Vol. 240, No. 1.
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abstract = "229 Th is the only nucleus currently under investigation for the development of a nuclear optical clock (NOC) of ultra-high accuracy. The insufficient knowledge of the first nuclear excitation energy of 229 Th has so far hindered direct nuclear laser spectroscopy of thorium ions and thus the development of a NOC. Here, a nuclear laser excitation scheme is detailed, which makes use of thorium atoms instead of ions. This concept, besides potentially leading to the first nuclear laser spectroscopy, would determine the isomeric energy to 40 μeV resolution, corresponding to 10 GHz, which is a 10 4 times improvement compared to the current best energy constraint. This would determine the nuclear isomeric energy to a sufficient accuracy to allow for nuclear laser spectroscopy of individual thorium ions in a Paul trap and thus the development of a single-ion nuclear optical clock. ",
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AU - von der Wense, Lars C.

AU - Seiferle, Benedict

AU - Schneider, Christian

AU - Jeet, Justin

AU - Amersdorffer, Ines

AU - Arlt, Nicolas

AU - Zacherl, Florian

AU - Haas, Raphael

AU - Renisch, Dennis

AU - Mosel, Patrick

AU - Mosel, Philip

AU - Kovacev, Milutin

AU - Morgner, Uwe

AU - Düllmann, Christoph E.

AU - Hudson, Eric R.

AU - Thirolf, Peter G.

N1 - Funding Information: Acknowledgements We would like to thank S. Stellmer and T. Schumm for discussions and lending of the VUV excimer laser. For discussions we are also grateful to G. Kazakov, A. Pálffy, J. Weitenberg and E. Peik. This work was supported by DFG (Th956/3-2) and by the European Union’s Horizon 2020 research and innovation programme under grant agreement 6674732 ”nuClock”. The efforts at UCLA have been supported in part by DARPA (QuASAR program), ARO (W911NF-11-1-0369), NSF (PHY-1205311), NIST PMG (60NANB14D302), RCSA (20112810), and DOE Office of Nuclear Physics, Isotope Programme.

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Y1 - 2019/3/13

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JO - Hyperfine Interactions

JF - Hyperfine Interactions

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ER -

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