Temperature dependence of the band gap of Si 28:P at very low temperatures measured via time-resolved optical spectroscopy

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Original languageEnglish
Article number013182
Number of pages10
JournalPhysical Review Research
Volume5
Issue number1
Publication statusPublished - 15 Mar 2023

Abstract

We measure the temperature dependence of the indirect band gap of isotopically purified Si28:P in the regime from 0.1 K to 3 K by high-resolution absorption spectroscopy of the donor bound exciton transition. The measurements increase the up-to-date precision of the temperature-dependent band gap change by more than one order of magnitude and reveal a T4 dependence which is about a factor of two less than observed in previous measurements. Such a T4 dependence is predicted by theory, but the absolute values differ between our experiment and the most up-to-date calculations by a factor of 30, corroborating that the electron-phonon interaction at low temperatures is still not correctly included into theory. What is more, the ability of such very high-precision band-gap measurements facilitates the use of time- and spatially resolved Si28:P absorption as a contactless, local thermometer and electric field sensor with a demonstrated time resolution of milliseconds.

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Temperature dependence of the band gap of Si 28:P at very low temperatures measured via time-resolved optical spectroscopy. / Sauter, E.; Abrosimov, N. V.; Hübner, J. et al.
In: Physical Review Research, Vol. 5, No. 1, 013182, 15.03.2023.

Research output: Contribution to journalArticleResearchpeer review

Sauter E, Abrosimov NV, Hübner J, Oestreich M. Temperature dependence of the band gap of Si 28:P at very low temperatures measured via time-resolved optical spectroscopy. Physical Review Research. 2023 Mar 15;5(1):013182. doi: 10.1103/PhysRevResearch.5.013182
Sauter, E. ; Abrosimov, N. V. ; Hübner, J. et al. / Temperature dependence of the band gap of Si 28:P at very low temperatures measured via time-resolved optical spectroscopy. In: Physical Review Research. 2023 ; Vol. 5, No. 1.
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title = "Temperature dependence of the band gap of Si 28:P at very low temperatures measured via time-resolved optical spectroscopy",
abstract = "We measure the temperature dependence of the indirect band gap of isotopically purified Si28:P in the regime from 0.1 K to 3 K by high-resolution absorption spectroscopy of the donor bound exciton transition. The measurements increase the up-to-date precision of the temperature-dependent band gap change by more than one order of magnitude and reveal a T4 dependence which is about a factor of two less than observed in previous measurements. Such a T4 dependence is predicted by theory, but the absolute values differ between our experiment and the most up-to-date calculations by a factor of 30, corroborating that the electron-phonon interaction at low temperatures is still not correctly included into theory. What is more, the ability of such very high-precision band-gap measurements facilitates the use of time- and spatially resolved Si28:P absorption as a contactless, local thermometer and electric field sensor with a demonstrated time resolution of milliseconds.",
author = "E. Sauter and Abrosimov, {N. V.} and J. H{\"u}bner and M. Oestreich",
note = "Funding Information: This work was funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy - EXC-2123 QuantumFrontiers - 390837967, Research Training Group 1991, OE-177/10-2, and OE-177/12-1. ",
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AU - Sauter, E.

AU - Abrosimov, N. V.

AU - Hübner, J.

AU - Oestreich, M.

N1 - Funding Information: This work was funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy - EXC-2123 QuantumFrontiers - 390837967, Research Training Group 1991, OE-177/10-2, and OE-177/12-1.

PY - 2023/3/15

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N2 - We measure the temperature dependence of the indirect band gap of isotopically purified Si28:P in the regime from 0.1 K to 3 K by high-resolution absorption spectroscopy of the donor bound exciton transition. The measurements increase the up-to-date precision of the temperature-dependent band gap change by more than one order of magnitude and reveal a T4 dependence which is about a factor of two less than observed in previous measurements. Such a T4 dependence is predicted by theory, but the absolute values differ between our experiment and the most up-to-date calculations by a factor of 30, corroborating that the electron-phonon interaction at low temperatures is still not correctly included into theory. What is more, the ability of such very high-precision band-gap measurements facilitates the use of time- and spatially resolved Si28:P absorption as a contactless, local thermometer and electric field sensor with a demonstrated time resolution of milliseconds.

AB - We measure the temperature dependence of the indirect band gap of isotopically purified Si28:P in the regime from 0.1 K to 3 K by high-resolution absorption spectroscopy of the donor bound exciton transition. The measurements increase the up-to-date precision of the temperature-dependent band gap change by more than one order of magnitude and reveal a T4 dependence which is about a factor of two less than observed in previous measurements. Such a T4 dependence is predicted by theory, but the absolute values differ between our experiment and the most up-to-date calculations by a factor of 30, corroborating that the electron-phonon interaction at low temperatures is still not correctly included into theory. What is more, the ability of such very high-precision band-gap measurements facilitates the use of time- and spatially resolved Si28:P absorption as a contactless, local thermometer and electric field sensor with a demonstrated time resolution of milliseconds.

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