Spin relaxation and spin-dependent exciton interactions in ZnSe quantum wells

Research output: Contribution to journalConference articleResearchpeer review

Authors

  • H. Kalt
  • J. Hoffmann
  • D. Tröndle
  • S. Wachter
  • D. Lüerßen
  • Daniel Hägele
  • W. W. Rühle
  • Michael Oestreich
  • I. J. Blewett
  • I. Galbraith

External Research Organisations

  • Karlsruhe Institute of Technology (KIT)
  • Philipps-Universität Marburg
  • Heriot-Watt University
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Details

Original languageEnglish
Pages (from-to)630-633
Number of pages4
JournalJournal of Crystal Growth
Volume214
Publication statusPublished - 2 Jun 2000
Externally publishedYes
EventThe 9th International Conference on II-VI Compounds - Kyoto, Jpn
Duration: 1 Nov 19995 Nov 1999

Abstract

We demonstrate the mutual influence of the dynamics in the real-space and the spin parts of the exciton wavefunction evoked by the exchange interaction. In the regime of high exciton density, the exciton-exciton interaction in ZnSe/ZnMgSSe quantum wells is found to be strongly affected by the exciton spin orientation and the longitudinal spin relaxation via single-fermion spin flips. The exciton's homogeneous linewidth as deduced from degenerate four-wave mixing with prepulse is significantly enhanced in spin-pure exciton populations by scattering including fermionic exchange. The transverse spin relaxation in the low-density limit is deduced from the decay of spin quantum-beats in photoluminescence experiments. We find an anti-proportionality between the spin relaxation and the optical dephasing times. The temperature dependence of both relaxation times is determined by the exciton-phonon interaction. The latter gradually reduces the electron-hole exchange coupling which is the dominating term in the exciton's transverse spin relaxation.

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Cite this

Spin relaxation and spin-dependent exciton interactions in ZnSe quantum wells. / Kalt, H.; Hoffmann, J.; Tröndle, D. et al.
In: Journal of Crystal Growth, Vol. 214, 02.06.2000, p. 630-633.

Research output: Contribution to journalConference articleResearchpeer review

Kalt, H, Hoffmann, J, Tröndle, D, Wachter, S, Lüerßen, D, Hägele, D, Rühle, WW, Oestreich, M, Blewett, IJ & Galbraith, I 2000, 'Spin relaxation and spin-dependent exciton interactions in ZnSe quantum wells', Journal of Crystal Growth, vol. 214, pp. 630-633. https://doi.org/10.1016/S0022-0248(00)00167-6
Kalt, H., Hoffmann, J., Tröndle, D., Wachter, S., Lüerßen, D., Hägele, D., Rühle, W. W., Oestreich, M., Blewett, I. J., & Galbraith, I. (2000). Spin relaxation and spin-dependent exciton interactions in ZnSe quantum wells. Journal of Crystal Growth, 214, 630-633. https://doi.org/10.1016/S0022-0248(00)00167-6
Kalt H, Hoffmann J, Tröndle D, Wachter S, Lüerßen D, Hägele D et al. Spin relaxation and spin-dependent exciton interactions in ZnSe quantum wells. Journal of Crystal Growth. 2000 Jun 2;214:630-633. doi: 10.1016/S0022-0248(00)00167-6
Kalt, H. ; Hoffmann, J. ; Tröndle, D. et al. / Spin relaxation and spin-dependent exciton interactions in ZnSe quantum wells. In: Journal of Crystal Growth. 2000 ; Vol. 214. pp. 630-633.
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TY - JOUR

T1 - Spin relaxation and spin-dependent exciton interactions in ZnSe quantum wells

AU - Kalt, H.

AU - Hoffmann, J.

AU - Tröndle, D.

AU - Wachter, S.

AU - Lüerßen, D.

AU - Hägele, Daniel

AU - Rühle, W. W.

AU - Oestreich, Michael

AU - Blewett, I. J.

AU - Galbraith, I.

PY - 2000/6/2

Y1 - 2000/6/2

N2 - We demonstrate the mutual influence of the dynamics in the real-space and the spin parts of the exciton wavefunction evoked by the exchange interaction. In the regime of high exciton density, the exciton-exciton interaction in ZnSe/ZnMgSSe quantum wells is found to be strongly affected by the exciton spin orientation and the longitudinal spin relaxation via single-fermion spin flips. The exciton's homogeneous linewidth as deduced from degenerate four-wave mixing with prepulse is significantly enhanced in spin-pure exciton populations by scattering including fermionic exchange. The transverse spin relaxation in the low-density limit is deduced from the decay of spin quantum-beats in photoluminescence experiments. We find an anti-proportionality between the spin relaxation and the optical dephasing times. The temperature dependence of both relaxation times is determined by the exciton-phonon interaction. The latter gradually reduces the electron-hole exchange coupling which is the dominating term in the exciton's transverse spin relaxation.

AB - We demonstrate the mutual influence of the dynamics in the real-space and the spin parts of the exciton wavefunction evoked by the exchange interaction. In the regime of high exciton density, the exciton-exciton interaction in ZnSe/ZnMgSSe quantum wells is found to be strongly affected by the exciton spin orientation and the longitudinal spin relaxation via single-fermion spin flips. The exciton's homogeneous linewidth as deduced from degenerate four-wave mixing with prepulse is significantly enhanced in spin-pure exciton populations by scattering including fermionic exchange. The transverse spin relaxation in the low-density limit is deduced from the decay of spin quantum-beats in photoluminescence experiments. We find an anti-proportionality between the spin relaxation and the optical dephasing times. The temperature dependence of both relaxation times is determined by the exciton-phonon interaction. The latter gradually reduces the electron-hole exchange coupling which is the dominating term in the exciton's transverse spin relaxation.

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U2 - 10.1016/S0022-0248(00)00167-6

DO - 10.1016/S0022-0248(00)00167-6

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AN - SCOPUS:17744402010

VL - 214

SP - 630

EP - 633

JO - Journal of Crystal Growth

JF - Journal of Crystal Growth

SN - 0022-0248

T2 - The 9th International Conference on II-VI Compounds

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