Solute transport in heterogeneous soil with time-dependent boundary conditions

Research output: Contribution to journalArticleResearchpeer review

Authors

  • Clemens J.M. Cremer
  • Insa Neuweiler
  • Michel Bechtold
  • Jan Vanderborght

External Research Organisations

  • Johann Heinrich von Thünen Institute, Federal Research Institute for Rural Areas, Forestry and Fisheries
  • Forschungszentrum Jülich
View graph of relations

Details

Original languageEnglish
Pages (from-to)1-17
JournalVadose zone journal
Volume15
Issue number6
Publication statusPublished - 17 Jun 2016

Abstract

We investigate the effect of dynamic boundary conditions on solute transport in unsaturated, heterogeneous, bimodal porous media. Solute transport is studied with two-dimensional numerical flow and transport models for scenarios where either (i) solely infiltration or (ii) more realistic dynamic (infiltration– evaporation) boundary conditions are imposed at the soil surface. Travel times of solute are affected by duration and intensity of infiltration and evaporation events even when cycle-averaged inflow rates of the scenarios are identical. Three main transport mechanisms could be identified based on a criterion for the infiltration rate that is related to the hydraulic conductivity curves of the media. If, based on this criterion, infiltration rates are low, the transport paths for upward and downward transport do not differ significantly, and the breakthrough curves of solute are similar to the one obtained under stationary infiltration. If infiltration rates are moderate, travel paths deviate between upward and downward flow, leading to a trapping of solute and strong tailing of the breakthrough curves. If infiltration and evaporation rates are very high, lateral advective–diffusive transport can lead to very efficient and fast downward transport. Thus, solute breakthrough depends strongly on lateral flow paths enforced by the boundary conditions at the soil surface. If heterogeneity of the materials is not strong and the structure is tortuous, dynamic boundary conditions mainly lead to increased macrodispersion. We test simplified upscaled transport models based on stationary flow rates to estimate breakthrough curves and demonstrate how the transport mechanisms are captured in the model parameters.

ASJC Scopus subject areas

Cite this

Solute transport in heterogeneous soil with time-dependent boundary conditions. / Cremer, Clemens J.M.; Neuweiler, Insa; Bechtold, Michel et al.
In: Vadose zone journal, Vol. 15, No. 6, 17.06.2016, p. 1-17.

Research output: Contribution to journalArticleResearchpeer review

Cremer, CJM, Neuweiler, I, Bechtold, M & Vanderborght, J 2016, 'Solute transport in heterogeneous soil with time-dependent boundary conditions', Vadose zone journal, vol. 15, no. 6, pp. 1-17. https://doi.org/10.2136/vzj2015.11.0144
Cremer, C. J. M., Neuweiler, I., Bechtold, M., & Vanderborght, J. (2016). Solute transport in heterogeneous soil with time-dependent boundary conditions. Vadose zone journal, 15(6), 1-17. https://doi.org/10.2136/vzj2015.11.0144
Cremer CJM, Neuweiler I, Bechtold M, Vanderborght J. Solute transport in heterogeneous soil with time-dependent boundary conditions. Vadose zone journal. 2016 Jun 17;15(6):1-17. doi: 10.2136/vzj2015.11.0144
Cremer, Clemens J.M. ; Neuweiler, Insa ; Bechtold, Michel et al. / Solute transport in heterogeneous soil with time-dependent boundary conditions. In: Vadose zone journal. 2016 ; Vol. 15, No. 6. pp. 1-17.
Download
@article{a77d306d1cb947cea1db150c2085a1e1,
title = "Solute transport in heterogeneous soil with time-dependent boundary conditions",
abstract = "We investigate the effect of dynamic boundary conditions on solute transport in unsaturated, heterogeneous, bimodal porous media. Solute transport is studied with two-dimensional numerical flow and transport models for scenarios where either (i) solely infiltration or (ii) more realistic dynamic (infiltration– evaporation) boundary conditions are imposed at the soil surface. Travel times of solute are affected by duration and intensity of infiltration and evaporation events even when cycle-averaged inflow rates of the scenarios are identical. Three main transport mechanisms could be identified based on a criterion for the infiltration rate that is related to the hydraulic conductivity curves of the media. If, based on this criterion, infiltration rates are low, the transport paths for upward and downward transport do not differ significantly, and the breakthrough curves of solute are similar to the one obtained under stationary infiltration. If infiltration rates are moderate, travel paths deviate between upward and downward flow, leading to a trapping of solute and strong tailing of the breakthrough curves. If infiltration and evaporation rates are very high, lateral advective–diffusive transport can lead to very efficient and fast downward transport. Thus, solute breakthrough depends strongly on lateral flow paths enforced by the boundary conditions at the soil surface. If heterogeneity of the materials is not strong and the structure is tortuous, dynamic boundary conditions mainly lead to increased macrodispersion. We test simplified upscaled transport models based on stationary flow rates to estimate breakthrough curves and demonstrate how the transport mechanisms are captured in the model parameters.",
author = "Cremer, {Clemens J.M.} and Insa Neuweiler and Michel Bechtold and Jan Vanderborght",
note = "This work was conducted in the context of the DFG Project FOR 1083 (NE 824/6–2): MUSIS (Multiscale Interfaces in Unsaturated Soil). Therefore, the authors wish to thank the Deutsche Forschungsgesellschaft (DFG) for funding.",
year = "2016",
month = jun,
day = "17",
doi = "10.2136/vzj2015.11.0144",
language = "English",
volume = "15",
pages = "1--17",
journal = "Vadose zone journal",
issn = "1539-1663",
publisher = "Soil Science Society of America",
number = "6",

}

Download

TY - JOUR

T1 - Solute transport in heterogeneous soil with time-dependent boundary conditions

AU - Cremer, Clemens J.M.

AU - Neuweiler, Insa

AU - Bechtold, Michel

AU - Vanderborght, Jan

N1 - This work was conducted in the context of the DFG Project FOR 1083 (NE 824/6–2): MUSIS (Multiscale Interfaces in Unsaturated Soil). Therefore, the authors wish to thank the Deutsche Forschungsgesellschaft (DFG) for funding.

PY - 2016/6/17

Y1 - 2016/6/17

N2 - We investigate the effect of dynamic boundary conditions on solute transport in unsaturated, heterogeneous, bimodal porous media. Solute transport is studied with two-dimensional numerical flow and transport models for scenarios where either (i) solely infiltration or (ii) more realistic dynamic (infiltration– evaporation) boundary conditions are imposed at the soil surface. Travel times of solute are affected by duration and intensity of infiltration and evaporation events even when cycle-averaged inflow rates of the scenarios are identical. Three main transport mechanisms could be identified based on a criterion for the infiltration rate that is related to the hydraulic conductivity curves of the media. If, based on this criterion, infiltration rates are low, the transport paths for upward and downward transport do not differ significantly, and the breakthrough curves of solute are similar to the one obtained under stationary infiltration. If infiltration rates are moderate, travel paths deviate between upward and downward flow, leading to a trapping of solute and strong tailing of the breakthrough curves. If infiltration and evaporation rates are very high, lateral advective–diffusive transport can lead to very efficient and fast downward transport. Thus, solute breakthrough depends strongly on lateral flow paths enforced by the boundary conditions at the soil surface. If heterogeneity of the materials is not strong and the structure is tortuous, dynamic boundary conditions mainly lead to increased macrodispersion. We test simplified upscaled transport models based on stationary flow rates to estimate breakthrough curves and demonstrate how the transport mechanisms are captured in the model parameters.

AB - We investigate the effect of dynamic boundary conditions on solute transport in unsaturated, heterogeneous, bimodal porous media. Solute transport is studied with two-dimensional numerical flow and transport models for scenarios where either (i) solely infiltration or (ii) more realistic dynamic (infiltration– evaporation) boundary conditions are imposed at the soil surface. Travel times of solute are affected by duration and intensity of infiltration and evaporation events even when cycle-averaged inflow rates of the scenarios are identical. Three main transport mechanisms could be identified based on a criterion for the infiltration rate that is related to the hydraulic conductivity curves of the media. If, based on this criterion, infiltration rates are low, the transport paths for upward and downward transport do not differ significantly, and the breakthrough curves of solute are similar to the one obtained under stationary infiltration. If infiltration rates are moderate, travel paths deviate between upward and downward flow, leading to a trapping of solute and strong tailing of the breakthrough curves. If infiltration and evaporation rates are very high, lateral advective–diffusive transport can lead to very efficient and fast downward transport. Thus, solute breakthrough depends strongly on lateral flow paths enforced by the boundary conditions at the soil surface. If heterogeneity of the materials is not strong and the structure is tortuous, dynamic boundary conditions mainly lead to increased macrodispersion. We test simplified upscaled transport models based on stationary flow rates to estimate breakthrough curves and demonstrate how the transport mechanisms are captured in the model parameters.

UR - http://www.scopus.com/inward/record.url?scp=84975165612&partnerID=8YFLogxK

U2 - 10.2136/vzj2015.11.0144

DO - 10.2136/vzj2015.11.0144

M3 - Article

AN - SCOPUS:84975165612

VL - 15

SP - 1

EP - 17

JO - Vadose zone journal

JF - Vadose zone journal

SN - 1539-1663

IS - 6

ER -