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Role of orbital symmetry in high-order harmonic generation from aligned molecules

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Authors

  • R. De Nalda
  • E. Heesel
  • Manfred Lein
  • N. Hay

External Research Organisations

  • Imperial College London
  • Max Planck Institute for the Physics of Complex Systems
  • Instituto Nazionale per la Fisica della Materia
  • Spanish National Research Council (CSIC)
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Details

Original languageEnglish
Article number031804
Pages (from-to)031804-1-031804-4
JournalPhysical Review A - Atomic, Molecular, and Optical Physics
Volume69
Issue number3
Publication statusPublished - 17 Mar 2004
Externally publishedYes

Abstract

The high-order harmonic generation (HHG) from aligned molecules in CO 2 was investigated. The time-dependant Schrödinger equation was solved in the single-active-electron approximation for a doubly antisymmetric initial wave function. The ionization and HHG for fixed orientations of the molecular axis with respect to electric field, was also studied. The HGG spectra of CO2 were measured for different preferential orientations for the molecular ensemble. The results show that the symmetry of the molecular ground state got imprinted in the outcome of strong-field phenomena.

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Cite this

Role of orbital symmetry in high-order harmonic generation from aligned molecules. / De Nalda, R.; Heesel, E.; Lein, Manfred et al.
In: Physical Review A - Atomic, Molecular, and Optical Physics, Vol. 69, No. 3, 031804, 17.03.2004, p. 031804-1-031804-4.

Research output: Contribution to journalArticleResearchpeer review

De Nalda, R, Heesel, E, Lein, M, Hay, N, Velotta, R, Springate, E, Castillejo, M & Marangos, JP 2004, 'Role of orbital symmetry in high-order harmonic generation from aligned molecules', Physical Review A - Atomic, Molecular, and Optical Physics, vol. 69, no. 3, 031804, pp. 031804-1-031804-4. https://doi.org/10.1103/PhysRevA.69.031804
De Nalda, R., Heesel, E., Lein, M., Hay, N., Velotta, R., Springate, E., Castillejo, M., & Marangos, J. P. (2004). Role of orbital symmetry in high-order harmonic generation from aligned molecules. Physical Review A - Atomic, Molecular, and Optical Physics, 69(3), 031804-1-031804-4. Article 031804. https://doi.org/10.1103/PhysRevA.69.031804
De Nalda R, Heesel E, Lein M, Hay N, Velotta R, Springate E et al. Role of orbital symmetry in high-order harmonic generation from aligned molecules. Physical Review A - Atomic, Molecular, and Optical Physics. 2004 Mar 17;69(3):031804-1-031804-4. 031804. doi: 10.1103/PhysRevA.69.031804
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AU - De Nalda, R.

AU - Heesel, E.

AU - Lein, Manfred

AU - Hay, N.

AU - Velotta, R.

AU - Springate, E.

AU - Castillejo, M.

AU - Marangos, J. P.

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