Polarization anisotropy and valence band ordering in semipolar (112¯2) AlInN/GaN heterostructures

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Authors

  • Shawutijiang Sidikejiang
  • Philipp Henning
  • Uwe Rossow
  • Heiko Bremers
  • Ferdinand Scholz
  • Andreas Hangleiter
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Original languageEnglish
Article number045202
JournalPhysical Review B
Volume107
Issue number4
Publication statusPublished - 5 Jan 2023
Externally publishedYes

Abstract

Semipolar (112¯2) AlInN/GaN heterostructures on GaN templates were studied using photoluminescence (PL) spectroscopy both at 15 K and at room temperature. The polarization-resolved PL measurements revealed a dominant polarization along the [112¯3¯] c′ and a weaker signal along the [11¯00] m-direction, i.e., the two in-plane directions of the semipolar (112¯2) growth plane. We observed slightly different polarization degrees of 0.34±0.01, 0.25±0.02, and 0.20±0.01 at room temperature, respectively, depending on the degree of strain relaxation in the [11¯00] direction. From a theoretical model based on a k·p calculation, we find that the transition from the conduction band (CB) to the uppermost valence band (VB) is C for AlInN similar to AlN, followed by the transition A from the CB to the second VB, for a wide range of compositions. Thus, the in-plane transition matrix elements from the CB to the two topmost VBs near the Γ point of the Brillouin zone are dominated by M[112¯3¯] for the C transition and by M[11¯00] for the A transition. For the samples under consideration with an energy splitting of about 18±1meV, there is sizable thermal occupation of the second VB at room temperature, reasonably explaining the experimental results. The results show that AlInN possesses a band structure similar to AlN, which might explain the strong Stokes shift and the large variation in the band-gap values reported previously.

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Cite this

Polarization anisotropy and valence band ordering in semipolar (112¯2) AlInN/GaN heterostructures. / Sidikejiang, Shawutijiang; Henning, Philipp; Rossow, Uwe et al.
In: Physical Review B, Vol. 107, No. 4, 045202, 05.01.2023.

Research output: Contribution to journalArticleResearchpeer review

Sidikejiang, S, Henning, P, Rossow, U, Bremers, H, Scholz, F & Hangleiter, A 2023, 'Polarization anisotropy and valence band ordering in semipolar (112¯2) AlInN/GaN heterostructures', Physical Review B, vol. 107, no. 4, 045202. https://doi.org/10.1103/physrevb.107.045202
Sidikejiang, S., Henning, P., Rossow, U., Bremers, H., Scholz, F., & Hangleiter, A. (2023). Polarization anisotropy and valence band ordering in semipolar (112¯2) AlInN/GaN heterostructures. Physical Review B, 107(4), Article 045202. https://doi.org/10.1103/physrevb.107.045202
Sidikejiang S, Henning P, Rossow U, Bremers H, Scholz F, Hangleiter A. Polarization anisotropy and valence band ordering in semipolar (112¯2) AlInN/GaN heterostructures. Physical Review B. 2023 Jan 5;107(4):045202. doi: 10.1103/physrevb.107.045202
Sidikejiang, Shawutijiang ; Henning, Philipp ; Rossow, Uwe et al. / Polarization anisotropy and valence band ordering in semipolar (112¯2) AlInN/GaN heterostructures. In: Physical Review B. 2023 ; Vol. 107, No. 4.
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abstract = "Semipolar (112¯2) AlInN/GaN heterostructures on GaN templates were studied using photoluminescence (PL) spectroscopy both at 15 K and at room temperature. The polarization-resolved PL measurements revealed a dominant polarization along the [112¯3¯] c′ and a weaker signal along the [11¯00] m-direction, i.e., the two in-plane directions of the semipolar (112¯2) growth plane. We observed slightly different polarization degrees of 0.34±0.01, 0.25±0.02, and 0.20±0.01 at room temperature, respectively, depending on the degree of strain relaxation in the [11¯00] direction. From a theoretical model based on a k·p calculation, we find that the transition from the conduction band (CB) to the uppermost valence band (VB) is C for AlInN similar to AlN, followed by the transition A from the CB to the second VB, for a wide range of compositions. Thus, the in-plane transition matrix elements from the CB to the two topmost VBs near the Γ point of the Brillouin zone are dominated by M[112¯3¯] for the C transition and by M[11¯00] for the A transition. For the samples under consideration with an energy splitting of about 18±1meV, there is sizable thermal occupation of the second VB at room temperature, reasonably explaining the experimental results. The results show that AlInN possesses a band structure similar to AlN, which might explain the strong Stokes shift and the large variation in the band-gap values reported previously.",
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AU - Sidikejiang, Shawutijiang

AU - Henning, Philipp

AU - Rossow, Uwe

AU - Bremers, Heiko

AU - Scholz, Ferdinand

AU - Hangleiter, Andreas

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N2 - Semipolar (112¯2) AlInN/GaN heterostructures on GaN templates were studied using photoluminescence (PL) spectroscopy both at 15 K and at room temperature. The polarization-resolved PL measurements revealed a dominant polarization along the [112¯3¯] c′ and a weaker signal along the [11¯00] m-direction, i.e., the two in-plane directions of the semipolar (112¯2) growth plane. We observed slightly different polarization degrees of 0.34±0.01, 0.25±0.02, and 0.20±0.01 at room temperature, respectively, depending on the degree of strain relaxation in the [11¯00] direction. From a theoretical model based on a k·p calculation, we find that the transition from the conduction band (CB) to the uppermost valence band (VB) is C for AlInN similar to AlN, followed by the transition A from the CB to the second VB, for a wide range of compositions. Thus, the in-plane transition matrix elements from the CB to the two topmost VBs near the Γ point of the Brillouin zone are dominated by M[112¯3¯] for the C transition and by M[11¯00] for the A transition. For the samples under consideration with an energy splitting of about 18±1meV, there is sizable thermal occupation of the second VB at room temperature, reasonably explaining the experimental results. The results show that AlInN possesses a band structure similar to AlN, which might explain the strong Stokes shift and the large variation in the band-gap values reported previously.

AB - Semipolar (112¯2) AlInN/GaN heterostructures on GaN templates were studied using photoluminescence (PL) spectroscopy both at 15 K and at room temperature. The polarization-resolved PL measurements revealed a dominant polarization along the [112¯3¯] c′ and a weaker signal along the [11¯00] m-direction, i.e., the two in-plane directions of the semipolar (112¯2) growth plane. We observed slightly different polarization degrees of 0.34±0.01, 0.25±0.02, and 0.20±0.01 at room temperature, respectively, depending on the degree of strain relaxation in the [11¯00] direction. From a theoretical model based on a k·p calculation, we find that the transition from the conduction band (CB) to the uppermost valence band (VB) is C for AlInN similar to AlN, followed by the transition A from the CB to the second VB, for a wide range of compositions. Thus, the in-plane transition matrix elements from the CB to the two topmost VBs near the Γ point of the Brillouin zone are dominated by M[112¯3¯] for the C transition and by M[11¯00] for the A transition. For the samples under consideration with an energy splitting of about 18±1meV, there is sizable thermal occupation of the second VB at room temperature, reasonably explaining the experimental results. The results show that AlInN possesses a band structure similar to AlN, which might explain the strong Stokes shift and the large variation in the band-gap values reported previously.

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