Photon bound state dynamics from a single artificial atom

Research output: Contribution to journalArticleResearchpeer review

Authors

  • Natasha Tomm
  • Sahand Mahmoodian
  • Nadia O. Antoniadis
  • Rüdiger Schott
  • Sascha R. Valentin
  • Andreas D. Wieck
  • Arne Ludwig
  • Alisa Javadi
  • Richard J. Warburton

Research Organisations

External Research Organisations

  • University of Basel
  • University of Sydney
  • Ruhr-Universität Bochum
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Details

Original languageEnglish
Pages (from-to)857-862
Number of pages6
JournalNature physics
Volume19
Issue number6
Early online date20 Mar 2023
Publication statusPublished - Jun 2023

Abstract

The interaction between photons and a single two-level atom constitutes a fundamental paradigm in quantum physics. The nonlinearity provided by the atom leads to a strong dependence of the light–matter interface on the number of photons interacting with the two-level system within its emission lifetime. This nonlinearity unveils strongly correlated quasiparticles known as photon bound states, giving rise to key physical processes such as stimulated emission and soliton propagation. Although signatures consistent with the existence of photon bound states have been measured in strongly interacting Rydberg gases, their hallmark excitation-number-dependent dispersion and propagation velocity have not yet been observed. Here we report the direct observation of a photon-number-dependent time delay in the scattering off a single artificial atom—a semiconductor quantum dot coupled to an optical cavity. By scattering a weak coherent pulse off the cavity–quantum electrodynamics system and measuring the time-dependent output power and correlation functions, we show that single photons and two- and three-photon bound states incur different time delays, becoming shorter for higher photon numbers. This reduced time delay is a fingerprint of stimulated emission, where the arrival of two photons within the lifetime of an emitter causes one photon to stimulate the emission of another.

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Cite this

Photon bound state dynamics from a single artificial atom. / Tomm, Natasha; Mahmoodian, Sahand; Antoniadis, Nadia O. et al.
In: Nature physics, Vol. 19, No. 6, 06.2023, p. 857-862.

Research output: Contribution to journalArticleResearchpeer review

Tomm, N, Mahmoodian, S, Antoniadis, NO, Schott, R, Valentin, SR, Wieck, AD, Ludwig, A, Javadi, A & Warburton, RJ 2023, 'Photon bound state dynamics from a single artificial atom', Nature physics, vol. 19, no. 6, pp. 857-862. https://doi.org/10.48550/arXiv.2205.03309, https://doi.org/10.1038/s41567-023-01997-6
Tomm, N., Mahmoodian, S., Antoniadis, N. O., Schott, R., Valentin, S. R., Wieck, A. D., Ludwig, A., Javadi, A., & Warburton, R. J. (2023). Photon bound state dynamics from a single artificial atom. Nature physics, 19(6), 857-862. https://doi.org/10.48550/arXiv.2205.03309, https://doi.org/10.1038/s41567-023-01997-6
Tomm N, Mahmoodian S, Antoniadis NO, Schott R, Valentin SR, Wieck AD et al. Photon bound state dynamics from a single artificial atom. Nature physics. 2023 Jun;19(6):857-862. Epub 2023 Mar 20. doi: 10.48550/arXiv.2205.03309, 10.1038/s41567-023-01997-6
Tomm, Natasha ; Mahmoodian, Sahand ; Antoniadis, Nadia O. et al. / Photon bound state dynamics from a single artificial atom. In: Nature physics. 2023 ; Vol. 19, No. 6. pp. 857-862.
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title = "Photon bound state dynamics from a single artificial atom",
abstract = "The interaction between photons and a single two-level atom constitutes a fundamental paradigm in quantum physics. The nonlinearity provided by the atom leads to a strong dependence of the light–matter interface on the number of photons interacting with the two-level system within its emission lifetime. This nonlinearity unveils strongly correlated quasiparticles known as photon bound states, giving rise to key physical processes such as stimulated emission and soliton propagation. Although signatures consistent with the existence of photon bound states have been measured in strongly interacting Rydberg gases, their hallmark excitation-number-dependent dispersion and propagation velocity have not yet been observed. Here we report the direct observation of a photon-number-dependent time delay in the scattering off a single artificial atom—a semiconductor quantum dot coupled to an optical cavity. By scattering a weak coherent pulse off the cavity–quantum electrodynamics system and measuring the time-dependent output power and correlation functions, we show that single photons and two- and three-photon bound states incur different time delays, becoming shorter for higher photon numbers. This reduced time delay is a fingerprint of stimulated emission, where the arrival of two photons within the lifetime of an emitter causes one photon to stimulate the emission of another.",
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note = "Funding Information: We thank K. Hammerer for fruitful discussions. N.T., N.O.A., A.J. and R.J.W. acknowledge financial support from SNF project 200020_204069 and NCCR QSIT. A.J. acknowledges support from the European Union{\textquoteright}s Horizon 2020 Research and Innovation Programme under Marie Sk{\l}odowska-Curie grant agreement no. 840453 (HiFig), and the Research Fund of the University of Basel. S.R.V., R.S., A.L. and A.D.W. gratefully acknowledge support from DFH/UFA CDFA05-06, DFG TRR160, DFG project 383065199 and BMBF Q.Link.X project 16KISQ009. S.M. acknowledges support from the Australian Research Council (ARC) via the Future Fellowship, {\textquoteleft}Emergent many-body phenomena in engineered quantum optical systems{\textquoteright}, project no. FT200100844, as well as the ARC Centre of Excellence in Engineered Quantum Systems (EQuS), project no. CE17010000. S.M. also acknowledges funding from DFG through CRC 1227 DQ-mat, projects A05 and A06, and {\textquoteleft}Nieders{\"a}chsisches Vorab{\textquoteright} through the {\textquoteleft}Quantum- and Nano-Metrology (QUANOMET){\textquoteright}. ",
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AU - Tomm, Natasha

AU - Mahmoodian, Sahand

AU - Antoniadis, Nadia O.

AU - Schott, Rüdiger

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AU - Ludwig, Arne

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N1 - Funding Information: We thank K. Hammerer for fruitful discussions. N.T., N.O.A., A.J. and R.J.W. acknowledge financial support from SNF project 200020_204069 and NCCR QSIT. A.J. acknowledges support from the European Union’s Horizon 2020 Research and Innovation Programme under Marie Skłodowska-Curie grant agreement no. 840453 (HiFig), and the Research Fund of the University of Basel. S.R.V., R.S., A.L. and A.D.W. gratefully acknowledge support from DFH/UFA CDFA05-06, DFG TRR160, DFG project 383065199 and BMBF Q.Link.X project 16KISQ009. S.M. acknowledges support from the Australian Research Council (ARC) via the Future Fellowship, ‘Emergent many-body phenomena in engineered quantum optical systems’, project no. FT200100844, as well as the ARC Centre of Excellence in Engineered Quantum Systems (EQuS), project no. CE17010000. S.M. also acknowledges funding from DFG through CRC 1227 DQ-mat, projects A05 and A06, and ‘Niedersächsisches Vorab’ through the ‘Quantum- and Nano-Metrology (QUANOMET)’.

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