Observing the Coulomb shifts of ionization times in high-order harmonic generation

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Original languageEnglish
Article number063102
JournalPhysical Review A
Volume107
Issue number6
Publication statusPublished - 5 Jun 2023

Abstract

The Coulomb interaction between the active electron and the parent ion is inherent in high-order harmonic generation from laser-driven atoms, but it is often neglected in modeling the electron dynamics. For this reason, the pioneering measurement scheme based on orthogonally polarized two-color fields [reported in Nature (London) 485, 343 (2012)0028-083610.1038/nature11025], which is able to measure ionization and return times for the electron trajectories, does not reflect the time shifts caused by the Coulomb interaction. We introduce a simple Coulomb correction to the electron motion in the two-color scheme, leading to modified retrieval equations for the extraction of time information from the observables. We apply the modified equations to data calculated from simulations of the time-dependent Schrödinger equation and we show that the scheme effectively reveals the Coulomb shift of the ionization time.

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Observing the Coulomb shifts of ionization times in high-order harmonic generation. / Yue, Shengjun; Liu, Jin; Xue, Shan et al.
In: Physical Review A, Vol. 107, No. 6, 063102, 05.06.2023.

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Yue S, Liu J, Xue S, Du H, Lein M. Observing the Coulomb shifts of ionization times in high-order harmonic generation. Physical Review A. 2023 Jun 5;107(6):063102. doi: 10.1103/PhysRevA.107.063102
Yue, Shengjun ; Liu, Jin ; Xue, Shan et al. / Observing the Coulomb shifts of ionization times in high-order harmonic generation. In: Physical Review A. 2023 ; Vol. 107, No. 6.
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AU - Yue, Shengjun

AU - Liu, Jin

AU - Xue, Shan

AU - Du, Hongchuan

AU - Lein, Manfred

N1 - Funding Information: This work has been supported by the National Natural Science Foundation of China (Grants No. 12204209, No. 12274188, and No. 12064023).

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