Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators

Research output: Contribution to journal › Article › Research › peer review

Authors

  • Anna A. Popkova
  • Ilya M. Antropov
  • Gleb I. Tselikov
  • Georgy A. Ermolaev
  • Igor Ozerov
  • Roman V. Kirtaev
  • Sergey M. Novikov
  • Andrey B. Evlyukhin
  • Aleksey V. Arsenin
  • Vladimir O. Bessonov
  • Valentyn S. Volkov
  • Andrey A. Fedyanin

Research Organisations

External Research Organisations

  • Lomonosov Moscow State University
  • Universite d'Aix-Marseille
  • GrapheneTek LLC
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Details

Original languageEnglish
Article number2100604
JournalLaser & photonics reviews
Volume16
Issue number6
Publication statusPublished - 15 Jun 2022

Abstract

Thanks to a high refractive index, giant optical anisotropy, and pronounced excitonic response, bulk transition metal dichalcogenides (TMDCs) have recently been discovered to be an ideal foundation for post-silicon photonics. The inversion symmetry of bulk TMDCs, on the other hand, prevents their use in nonlinear-optical processes such as second-harmonic generation (SHG). To overcome this obstacle and broaden the application scope of TMDCs, MoS2 nanodisks are engineered to couple Mie resonances with C-excitons. As a result, their alliance produces 23-fold enhancement of SHG intensity with respect to the resonant SHG from a high-quality exfoliated MoS2 monolayer under C-exciton excitation. Furthermore, SHG demonstrates a strongly anisotropic response typical of a MoS2 monolayer due to the single-crystal structure of the fabricated nanodisks, providing a polarization degree of freedom to manipulate SHG. Hence, these results significantly improve the potential of bulk TMDCs enabling an avenue for next-generation nonlinear photonics.

Keywords

    excitons, Mie resonances, molybdenum disulfide, second-harmonic generation, transition metal dichalcogenides

ASJC Scopus subject areas

Cite this

Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators. / Popkova, Anna A.; Antropov, Ilya M.; Tselikov, Gleb I. et al.
In: Laser & photonics reviews, Vol. 16, No. 6, 2100604, 15.06.2022.

Research output: Contribution to journal › Article › Research › peer review

Popkova, AA, Antropov, IM, Tselikov, GI, Ermolaev, GA, Ozerov, I, Kirtaev, RV, Novikov, SM, Evlyukhin, AB, Arsenin, AV, Bessonov, VO, Volkov, VS & Fedyanin, AA 2022, 'Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators', Laser & photonics reviews, vol. 16, no. 6, 2100604. https://doi.org/10.1002/lpor.202100604
Popkova, A. A., Antropov, I. M., Tselikov, G. I., Ermolaev, G. A., Ozerov, I., Kirtaev, R. V., Novikov, S. M., Evlyukhin, A. B., Arsenin, A. V., Bessonov, V. O., Volkov, V. S., & Fedyanin, A. A. (2022). Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators. Laser & photonics reviews, 16(6), Article 2100604. https://doi.org/10.1002/lpor.202100604
Popkova AA, Antropov IM, Tselikov GI, Ermolaev GA, Ozerov I, Kirtaev RV et al. Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators. Laser & photonics reviews. 2022 Jun 15;16(6):2100604. doi: 10.1002/lpor.202100604
Popkova, Anna A. ; Antropov, Ilya M. ; Tselikov, Gleb I. et al. / Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators. In: Laser & photonics reviews. 2022 ; Vol. 16, No. 6.
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title = "Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators",
abstract = "Thanks to a high refractive index, giant optical anisotropy, and pronounced excitonic response, bulk transition metal dichalcogenides (TMDCs) have recently been discovered to be an ideal foundation for post-silicon photonics. The inversion symmetry of bulk TMDCs, on the other hand, prevents their use in nonlinear-optical processes such as second-harmonic generation (SHG). To overcome this obstacle and broaden the application scope of TMDCs, MoS2 nanodisks are engineered to couple Mie resonances with C-excitons. As a result, their alliance produces 23-fold enhancement of SHG intensity with respect to the resonant SHG from a high-quality exfoliated MoS2 monolayer under C-exciton excitation. Furthermore, SHG demonstrates a strongly anisotropic response typical of a MoS2 monolayer due to the single-crystal structure of the fabricated nanodisks, providing a polarization degree of freedom to manipulate SHG. Hence, these results significantly improve the potential of bulk TMDCs enabling an avenue for next-generation nonlinear photonics.",
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author = "Popkova, {Anna A.} and Antropov, {Ilya M.} and Tselikov, {Gleb I.} and Ermolaev, {Georgy A.} and Igor Ozerov and Kirtaev, {Roman V.} and Novikov, {Sergey M.} and Evlyukhin, {Andrey B.} and Arsenin, {Aleksey V.} and Bessonov, {Vladimir O.} and Volkov, {Valentyn S.} and Fedyanin, {Andrey A.}",
note = "Funding Information: The authors sincerely thank Fr{\'e}d{\'e}ric Bedu for his help with nanofabrication processes performed at PLANETE cleanroom facility (CINaM, Marseille). The work was performed under partial financial support of the Russian Ministry of Education and Science (Grant No. 14.W03.31.0008), the Russian Science Foundation (grant No. 21‐19‐00675, sample design and fabrication; grant No. 21‐79‐00206, linear optical characterization; grant No. 20‐12‐00371, nonlinear‐optical measurements), and Russian Foundation for Basic Research (grant No.21‐52‐12036, numerical simulations). Part of the research was supported by MSU Quantum Technology Centre and the Development program of the MSU Interdisciplinary Scientific and Educational School “Photonic and Quantum technologies. Digital Medicine”. The support from the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122, Project ID 390833453) is acknowledged. A.A.P. acknowledges support by “BASIS” Foundation (grant No. 19‐2‐6‐28‐1). G.A.E. acknowledges support by grant of the President of Russian Federation to young scientists and postgraduates.",
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T1 - Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators

AU - Popkova, Anna A.

AU - Antropov, Ilya M.

AU - Tselikov, Gleb I.

AU - Ermolaev, Georgy A.

AU - Ozerov, Igor

AU - Kirtaev, Roman V.

AU - Novikov, Sergey M.

AU - Evlyukhin, Andrey B.

AU - Arsenin, Aleksey V.

AU - Bessonov, Vladimir O.

AU - Volkov, Valentyn S.

AU - Fedyanin, Andrey A.

N1 - Funding Information: The authors sincerely thank Frédéric Bedu for his help with nanofabrication processes performed at PLANETE cleanroom facility (CINaM, Marseille). The work was performed under partial financial support of the Russian Ministry of Education and Science (Grant No. 14.W03.31.0008), the Russian Science Foundation (grant No. 21‐19‐00675, sample design and fabrication; grant No. 21‐79‐00206, linear optical characterization; grant No. 20‐12‐00371, nonlinear‐optical measurements), and Russian Foundation for Basic Research (grant No.21‐52‐12036, numerical simulations). Part of the research was supported by MSU Quantum Technology Centre and the Development program of the MSU Interdisciplinary Scientific and Educational School “Photonic and Quantum technologies. Digital Medicine”. The support from the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122, Project ID 390833453) is acknowledged. A.A.P. acknowledges support by “BASIS” Foundation (grant No. 19‐2‐6‐28‐1). G.A.E. acknowledges support by grant of the President of Russian Federation to young scientists and postgraduates.

PY - 2022/6/15

Y1 - 2022/6/15

N2 - Thanks to a high refractive index, giant optical anisotropy, and pronounced excitonic response, bulk transition metal dichalcogenides (TMDCs) have recently been discovered to be an ideal foundation for post-silicon photonics. The inversion symmetry of bulk TMDCs, on the other hand, prevents their use in nonlinear-optical processes such as second-harmonic generation (SHG). To overcome this obstacle and broaden the application scope of TMDCs, MoS2 nanodisks are engineered to couple Mie resonances with C-excitons. As a result, their alliance produces 23-fold enhancement of SHG intensity with respect to the resonant SHG from a high-quality exfoliated MoS2 monolayer under C-exciton excitation. Furthermore, SHG demonstrates a strongly anisotropic response typical of a MoS2 monolayer due to the single-crystal structure of the fabricated nanodisks, providing a polarization degree of freedom to manipulate SHG. Hence, these results significantly improve the potential of bulk TMDCs enabling an avenue for next-generation nonlinear photonics.

AB - Thanks to a high refractive index, giant optical anisotropy, and pronounced excitonic response, bulk transition metal dichalcogenides (TMDCs) have recently been discovered to be an ideal foundation for post-silicon photonics. The inversion symmetry of bulk TMDCs, on the other hand, prevents their use in nonlinear-optical processes such as second-harmonic generation (SHG). To overcome this obstacle and broaden the application scope of TMDCs, MoS2 nanodisks are engineered to couple Mie resonances with C-excitons. As a result, their alliance produces 23-fold enhancement of SHG intensity with respect to the resonant SHG from a high-quality exfoliated MoS2 monolayer under C-exciton excitation. Furthermore, SHG demonstrates a strongly anisotropic response typical of a MoS2 monolayer due to the single-crystal structure of the fabricated nanodisks, providing a polarization degree of freedom to manipulate SHG. Hence, these results significantly improve the potential of bulk TMDCs enabling an avenue for next-generation nonlinear photonics.

KW - excitons

KW - Mie resonances

KW - molybdenum disulfide

KW - second-harmonic generation

KW - transition metal dichalcogenides

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U2 - 10.1002/lpor.202100604

DO - 10.1002/lpor.202100604

M3 - Article

VL - 16

JO - Laser & photonics reviews

JF - Laser & photonics reviews

SN - 1863-8880

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M1 - 2100604

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