Magnetic-Field Effect in High-Order Above-Threshold Ionization

Research output: Contribution to journalArticleResearchpeer review

Authors

  • Kang Lin
  • Simon Brennecke
  • Hongcheng Ni
  • Xiang Chen
  • Alexander Hartung
  • Daniel Trabert
  • Kilian Fehre
  • Jonas Rist
  • Xiao Min Tong
  • Joachim Burgdörfer
  • Lothar Ph H. Schmidt
  • Markus S. Schöffler
  • Till Jahnke
  • Maksim Kunitski
  • Feng He
  • Manfred Lein
  • Sebastian Eckart
  • Reinhard Dörner

Research Organisations

External Research Organisations

  • Goethe University Frankfurt
  • East China Normal University
  • TU Wien (TUW)
  • Shanxi University
  • Shanghai Jiaotong University
  • University of Tsukuba
  • Chinese Academy of Sciences (CAS)
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Details

Original languageEnglish
Article number023201
JournalPhysical review letters
Volume128
Issue number2
Publication statusPublished - 14 Jan 2022

Abstract

We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift of the electron momentum distribution along the light-propagation direction for high energy electrons beyond the 2Up classical cutoff is found to be vastly different from that below this cutoff, where Up is the ponderomotive potential of the driving laser field. A local minimum structure in the momentum dependence of the nondipole shift above the cutoff is identified for the first time. With the help of classical and quantum-orbit analysis, we show that large-angle rescattering of the electrons strongly alters the partitioning of the photon momentum between electron and ion. The sensitivity of the observed nondipole shift to the electronic structure of the target atom is confirmed by three-dimensional time-dependent Schrödinger equation simulations for different model potentials. Our work paves the way toward understanding the physics of extreme light-matter interactions at long wavelengths and high electron kinetic energies.

ASJC Scopus subject areas

Cite this

Magnetic-Field Effect in High-Order Above-Threshold Ionization. / Lin, Kang; Brennecke, Simon; Ni, Hongcheng et al.
In: Physical review letters, Vol. 128, No. 2, 023201, 14.01.2022.

Research output: Contribution to journalArticleResearchpeer review

Lin, K, Brennecke, S, Ni, H, Chen, X, Hartung, A, Trabert, D, Fehre, K, Rist, J, Tong, XM, Burgdörfer, J, Schmidt, LPH, Schöffler, MS, Jahnke, T, Kunitski, M, He, F, Lein, M, Eckart, S & Dörner, R 2022, 'Magnetic-Field Effect in High-Order Above-Threshold Ionization', Physical review letters, vol. 128, no. 2, 023201. https://doi.org/10.48550/arXiv.2110.08601, https://doi.org/10.1103/PhysRevLett.128.023201
Lin, K., Brennecke, S., Ni, H., Chen, X., Hartung, A., Trabert, D., Fehre, K., Rist, J., Tong, X. M., Burgdörfer, J., Schmidt, L. P. H., Schöffler, M. S., Jahnke, T., Kunitski, M., He, F., Lein, M., Eckart, S., & Dörner, R. (2022). Magnetic-Field Effect in High-Order Above-Threshold Ionization. Physical review letters, 128(2), Article 023201. https://doi.org/10.48550/arXiv.2110.08601, https://doi.org/10.1103/PhysRevLett.128.023201
Lin K, Brennecke S, Ni H, Chen X, Hartung A, Trabert D et al. Magnetic-Field Effect in High-Order Above-Threshold Ionization. Physical review letters. 2022 Jan 14;128(2):023201. doi: 10.48550/arXiv.2110.08601, 10.1103/PhysRevLett.128.023201
Lin, Kang ; Brennecke, Simon ; Ni, Hongcheng et al. / Magnetic-Field Effect in High-Order Above-Threshold Ionization. In: Physical review letters. 2022 ; Vol. 128, No. 2.
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title = "Magnetic-Field Effect in High-Order Above-Threshold Ionization",
abstract = "We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift of the electron momentum distribution along the light-propagation direction for high energy electrons beyond the 2Up classical cutoff is found to be vastly different from that below this cutoff, where Up is the ponderomotive potential of the driving laser field. A local minimum structure in the momentum dependence of the nondipole shift above the cutoff is identified for the first time. With the help of classical and quantum-orbit analysis, we show that large-angle rescattering of the electrons strongly alters the partitioning of the photon momentum between electron and ion. The sensitivity of the observed nondipole shift to the electronic structure of the target atom is confirmed by three-dimensional time-dependent Schr{\"o}dinger equation simulations for different model potentials. Our work paves the way toward understanding the physics of extreme light-matter interactions at long wavelengths and high electron kinetic energies.",
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note = "Funding Information: The experimental work was supported by the DFG (German Research Foundation). K. L. acknowledges support by the Alexander von Humboldt Foundation and thanks Xiaoqing Hu and Wenbin Zhang for helpful discussions. S. E. acknowledges funding of the DFG through Priority Programme SPP 1840 QUTIF. A. H. and K. F. acknowledge support by the German Academic Scholarship Foundation. X. M. T. was supported by Multidisciplinary Cooperative Research Program in CCS, University of Tsukuba. F. H. acknowledges the support by the National Science Foundation of China (No. 11925405). H. N. acknowledges the support by Project No. 11904103 of the National Natural Science Foundation of China (NSFC), Project No. M2692 of the Austrian Science Fund (FWF), and Projects No. 21ZR1420100 and No. 19JC1412200 of the Science and Technology Commission of Shanghai Municipality. Numerical simulations were in part performed on the East China Normal University (ECNU) Multifunctional Platform for Innovation (001). ",
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Download

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T1 - Magnetic-Field Effect in High-Order Above-Threshold Ionization

AU - Lin, Kang

AU - Brennecke, Simon

AU - Ni, Hongcheng

AU - Chen, Xiang

AU - Hartung, Alexander

AU - Trabert, Daniel

AU - Fehre, Kilian

AU - Rist, Jonas

AU - Tong, Xiao Min

AU - Burgdörfer, Joachim

AU - Schmidt, Lothar Ph H.

AU - Schöffler, Markus S.

AU - Jahnke, Till

AU - Kunitski, Maksim

AU - He, Feng

AU - Lein, Manfred

AU - Eckart, Sebastian

AU - Dörner, Reinhard

N1 - Funding Information: The experimental work was supported by the DFG (German Research Foundation). K. L. acknowledges support by the Alexander von Humboldt Foundation and thanks Xiaoqing Hu and Wenbin Zhang for helpful discussions. S. E. acknowledges funding of the DFG through Priority Programme SPP 1840 QUTIF. A. H. and K. F. acknowledge support by the German Academic Scholarship Foundation. X. M. T. was supported by Multidisciplinary Cooperative Research Program in CCS, University of Tsukuba. F. H. acknowledges the support by the National Science Foundation of China (No. 11925405). H. N. acknowledges the support by Project No. 11904103 of the National Natural Science Foundation of China (NSFC), Project No. M2692 of the Austrian Science Fund (FWF), and Projects No. 21ZR1420100 and No. 19JC1412200 of the Science and Technology Commission of Shanghai Municipality. Numerical simulations were in part performed on the East China Normal University (ECNU) Multifunctional Platform for Innovation (001).

PY - 2022/1/14

Y1 - 2022/1/14

N2 - We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift of the electron momentum distribution along the light-propagation direction for high energy electrons beyond the 2Up classical cutoff is found to be vastly different from that below this cutoff, where Up is the ponderomotive potential of the driving laser field. A local minimum structure in the momentum dependence of the nondipole shift above the cutoff is identified for the first time. With the help of classical and quantum-orbit analysis, we show that large-angle rescattering of the electrons strongly alters the partitioning of the photon momentum between electron and ion. The sensitivity of the observed nondipole shift to the electronic structure of the target atom is confirmed by three-dimensional time-dependent Schrödinger equation simulations for different model potentials. Our work paves the way toward understanding the physics of extreme light-matter interactions at long wavelengths and high electron kinetic energies.

AB - We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift of the electron momentum distribution along the light-propagation direction for high energy electrons beyond the 2Up classical cutoff is found to be vastly different from that below this cutoff, where Up is the ponderomotive potential of the driving laser field. A local minimum structure in the momentum dependence of the nondipole shift above the cutoff is identified for the first time. With the help of classical and quantum-orbit analysis, we show that large-angle rescattering of the electrons strongly alters the partitioning of the photon momentum between electron and ion. The sensitivity of the observed nondipole shift to the electronic structure of the target atom is confirmed by three-dimensional time-dependent Schrödinger equation simulations for different model potentials. Our work paves the way toward understanding the physics of extreme light-matter interactions at long wavelengths and high electron kinetic energies.

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JO - Physical review letters

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SN - 0031-9007

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