Investigations in the nonlinear behavior of dielectrics by using ultrashort pulses

Research output: Chapter in book/report/conference proceedingConference contributionResearchpeer review

Authors

  • Kai Starke
  • Detlev Ristau
  • Herbert Welling
  • Tatiana Amotchkina
  • Michael K. Trubetskov
  • A. S. Chirkin
  • Andrei A. Tikhonravov

External Research Organisations

  • Laser Zentrum Hannover e.V. (LZH)
  • Lomonosov Moscow State University
View graph of relations

Details

Original languageEnglish
Title of host publicationLaser-Induced Damage in Optical Materials: 2003
Subtitle of host publication35th Annual Boulder Damage Symposium proceedings ; 22 - 24 September 2003, Boulder, Colorado
Place of PublicationBellingham
PublisherSPIE
Pages501-514
Number of pages14
ISBN (print)0-8194-5163-0
Publication statusPublished - 10 Jun 2004
Externally publishedYes
Event35th Annual Boulder Damage Symposium: Laser-Induced Damage in Optical Materials 2003 - Boulder, CO, United States
Duration: 22 Sept 200324 Sept 2003

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
PublisherSPIE
Volume5273
ISSN (Print)0277-786X

Abstract

Ultra-short pulse systems are considered as innovative laser sources for a variety of applications in micro material structuring, medicine and diagnostics. Current commercial systems are still lacking in output power limiting the throughput and the economic efficiency within a production line. In the optimization of ultra short pulse sources of the next generation, special effects in optical components during interaction with ultra-short pulses play a major role. Especially, low damage thresholds and non-linear absorptance have already been observed within the activities of the EUREKA-project CHOCLAB II, which are concentrated on the evaluation of multiple-pulse damage and the absorptance of fs-optical components according to the International Standards ISO 11254-2 and ISO 11551. In this paper, a theoretical model on the basis of photo- and avalanche ionization is presented describing the incidence of damage as a consequence of a sufficient high density of conduction band electrons. Furthermore, the influence of the Kerr-effect and conduction band electrons on the optical properties of dielectrics is investigated theoretically. From our calculations, a significant increase in reflectance due to the dominant Kerr-effect can be deduced as well as a noticeable increase in absorptance induced by free electron heating already at energy density values clearly below the damage threshold. Finally, results of an experimental investigation in the influence of the internal field strength in a dielectric layer stack on the damage threshold are described. The experiments clearly support the assumption already stated in other publications, that the field intensity formed by the optical design plays a key role for damage resistance of optical coatings for ultrashort pulses.

Keywords

    Avalanche-ionization, Critical electron density, Keldysh, Kerr-effect, Multiple-pulse damage threshold, Nonlinear absorptance, Ultrashort pulses

ASJC Scopus subject areas

Cite this

Investigations in the nonlinear behavior of dielectrics by using ultrashort pulses. / Starke, Kai; Ristau, Detlev; Welling, Herbert et al.
Laser-Induced Damage in Optical Materials: 2003: 35th Annual Boulder Damage Symposium proceedings ; 22 - 24 September 2003, Boulder, Colorado. Bellingham: SPIE, 2004. p. 501-514 (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 5273).

Research output: Chapter in book/report/conference proceedingConference contributionResearchpeer review

Starke, K, Ristau, D, Welling, H, Amotchkina, T, Trubetskov, MK, Chirkin, AS & Tikhonravov, AA 2004, Investigations in the nonlinear behavior of dielectrics by using ultrashort pulses. in Laser-Induced Damage in Optical Materials: 2003: 35th Annual Boulder Damage Symposium proceedings ; 22 - 24 September 2003, Boulder, Colorado. Proceedings of SPIE - The International Society for Optical Engineering, vol. 5273, SPIE, Bellingham, pp. 501-514, 35th Annual Boulder Damage Symposium, Boulder, CO, United States, 22 Sept 2003. https://doi.org/10.1117/12.525132
Starke, K., Ristau, D., Welling, H., Amotchkina, T., Trubetskov, M. K., Chirkin, A. S., & Tikhonravov, A. A. (2004). Investigations in the nonlinear behavior of dielectrics by using ultrashort pulses. In Laser-Induced Damage in Optical Materials: 2003: 35th Annual Boulder Damage Symposium proceedings ; 22 - 24 September 2003, Boulder, Colorado (pp. 501-514). (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 5273). SPIE. https://doi.org/10.1117/12.525132
Starke K, Ristau D, Welling H, Amotchkina T, Trubetskov MK, Chirkin AS et al. Investigations in the nonlinear behavior of dielectrics by using ultrashort pulses. In Laser-Induced Damage in Optical Materials: 2003: 35th Annual Boulder Damage Symposium proceedings ; 22 - 24 September 2003, Boulder, Colorado. Bellingham: SPIE. 2004. p. 501-514. (Proceedings of SPIE - The International Society for Optical Engineering). doi: 10.1117/12.525132
Starke, Kai ; Ristau, Detlev ; Welling, Herbert et al. / Investigations in the nonlinear behavior of dielectrics by using ultrashort pulses. Laser-Induced Damage in Optical Materials: 2003: 35th Annual Boulder Damage Symposium proceedings ; 22 - 24 September 2003, Boulder, Colorado. Bellingham : SPIE, 2004. pp. 501-514 (Proceedings of SPIE - The International Society for Optical Engineering).
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abstract = "Ultra-short pulse systems are considered as innovative laser sources for a variety of applications in micro material structuring, medicine and diagnostics. Current commercial systems are still lacking in output power limiting the throughput and the economic efficiency within a production line. In the optimization of ultra short pulse sources of the next generation, special effects in optical components during interaction with ultra-short pulses play a major role. Especially, low damage thresholds and non-linear absorptance have already been observed within the activities of the EUREKA-project CHOCLAB II, which are concentrated on the evaluation of multiple-pulse damage and the absorptance of fs-optical components according to the International Standards ISO 11254-2 and ISO 11551. In this paper, a theoretical model on the basis of photo- and avalanche ionization is presented describing the incidence of damage as a consequence of a sufficient high density of conduction band electrons. Furthermore, the influence of the Kerr-effect and conduction band electrons on the optical properties of dielectrics is investigated theoretically. From our calculations, a significant increase in reflectance due to the dominant Kerr-effect can be deduced as well as a noticeable increase in absorptance induced by free electron heating already at energy density values clearly below the damage threshold. Finally, results of an experimental investigation in the influence of the internal field strength in a dielectric layer stack on the damage threshold are described. The experiments clearly support the assumption already stated in other publications, that the field intensity formed by the optical design plays a key role for damage resistance of optical coatings for ultrashort pulses.",
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AU - Starke, Kai

AU - Ristau, Detlev

AU - Welling, Herbert

AU - Amotchkina, Tatiana

AU - Trubetskov, Michael K.

AU - Chirkin, A. S.

AU - Tikhonravov, Andrei A.

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