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Influence of nuclear vibration on harmonic generation in molecules

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  • Max Planck Institute for Nuclear Physics

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Original languageEnglish
Article numberS17
Pages (from-to)S437-S444
JournalJournal of Physics B: Atomic, Molecular and Optical Physics
Volume39
Issue number13
Publication statusPublished - 22 Jun 2006
Externally publishedYes

Abstract

The effect of vibrational motion on harmonic generation in molecules is studied within the strong-field approximation. Simple expressions are given for the cut-off energy and for the ratio of spectral intensities from two isotopes. The latter is based on electronic trajectories from the simple-man's model. The influence of vibration is given by a correlation function that is sensitive to the overlap between the initial vibrational wave packet and the wave packet after the evolution in the Born-Oppenheimer potential of the ionized molecule.

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Cite this

Influence of nuclear vibration on harmonic generation in molecules. / Chirilǎ, Ciprian C.; Lein, Manfred.
In: Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 39, No. 13, S17, 22.06.2006, p. S437-S444.

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