Gas Component Transport Across the Soil-Atmosphere Interface for Gases of Different Density: Experiments and Modeling

Research output: Contribution to journalArticleResearchpeer review

Authors

  • L. M. Bahlmann
  • K. M. Smits
  • K. Heck
  • E. Coltman
  • R. Helmig
  • I. Neuweiler

External Research Organisations

  • University of Texas at Arlington
  • University of Stuttgart
  • Colorado School of Mines (CSM)
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Details

Original languageEnglish
Article numbere2020WR027600
JournalWater resources research
Volume56
Issue number9
Early online date3 Aug 2020
Publication statusPublished - 1 Sept 2020

Abstract

We investigate the influence of near-surface wind conditions on subsurface gas transport and on soil-atmosphere gas exchange for gases of different density. Results of a sand tank experiment are supported by a numerical investigation with a fully coupled porous medium-free flow model, which accounts for wind turbulence. The experiment consists of a two-dimensional bench-scale soil tank containing homogeneous sand and an overlying wind tunnel. A point source was installed at the bottom of the tank. Gas concentrations were measured at multiple horizontal and vertical locations. Tested conditions include four wind velocities (0.2/1.0/2.0/2.7 m/s), three different gases (helium: light, nitrogen: neutral, and carbon dioxide: heavy), and two transport cases (1: steady-state gas supply from the point source; 2: transport under decreasing concentration gradient, subsequent to termination of gas supply). The model was used to assess flow patterns and gas fluxes across the soil surface. Results demonstrate that flow and transport in the vicinity of the surface are strongly coupled to the overlying wind field. An increase in wind velocity accelerates soil-atmosphere gas exchange. This is due to the effect of the wind profile on soil surface concentrations and due to wind-induced advection, which causes subsurface horizontal transport. The presence of gases with pronounced density difference to air adds additional complexity to the transport through the wind-affected soil layers. Wind impact differs between tested gases. Observed transport is multidimensional and shows that heavy as well as light gases cannot be treated as inert tracers, which applies to many gases in environmental studies.

Keywords

    density effects, gas component transport, numerical modeling, soil-atmosphere interface, wind-induced transport

ASJC Scopus subject areas

Cite this

Gas Component Transport Across the Soil-Atmosphere Interface for Gases of Different Density: Experiments and Modeling. / Bahlmann, L. M.; Smits, K. M.; Heck, K. et al.
In: Water resources research, Vol. 56, No. 9, e2020WR027600, 01.09.2020.

Research output: Contribution to journalArticleResearchpeer review

Bahlmann, L. M., Smits, K. M., Heck, K., Coltman, E., Helmig, R., & Neuweiler, I. (2020). Gas Component Transport Across the Soil-Atmosphere Interface for Gases of Different Density: Experiments and Modeling. Water resources research, 56(9), Article e2020WR027600. https://doi.org/10.1029/2020WR027600
Bahlmann LM, Smits KM, Heck K, Coltman E, Helmig R, Neuweiler I. Gas Component Transport Across the Soil-Atmosphere Interface for Gases of Different Density: Experiments and Modeling. Water resources research. 2020 Sept 1;56(9):e2020WR027600. Epub 2020 Aug 3. doi: 10.1029/2020WR027600
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title = "Gas Component Transport Across the Soil-Atmosphere Interface for Gases of Different Density: Experiments and Modeling",
abstract = "We investigate the influence of near-surface wind conditions on subsurface gas transport and on soil-atmosphere gas exchange for gases of different density. Results of a sand tank experiment are supported by a numerical investigation with a fully coupled porous medium-free flow model, which accounts for wind turbulence. The experiment consists of a two-dimensional bench-scale soil tank containing homogeneous sand and an overlying wind tunnel. A point source was installed at the bottom of the tank. Gas concentrations were measured at multiple horizontal and vertical locations. Tested conditions include four wind velocities (0.2/1.0/2.0/2.7 m/s), three different gases (helium: light, nitrogen: neutral, and carbon dioxide: heavy), and two transport cases (1: steady-state gas supply from the point source; 2: transport under decreasing concentration gradient, subsequent to termination of gas supply). The model was used to assess flow patterns and gas fluxes across the soil surface. Results demonstrate that flow and transport in the vicinity of the surface are strongly coupled to the overlying wind field. An increase in wind velocity accelerates soil-atmosphere gas exchange. This is due to the effect of the wind profile on soil surface concentrations and due to wind-induced advection, which causes subsurface horizontal transport. The presence of gases with pronounced density difference to air adds additional complexity to the transport through the wind-affected soil layers. Wind impact differs between tested gases. Observed transport is multidimensional and shows that heavy as well as light gases cannot be treated as inert tracers, which applies to many gases in environmental studies.",
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T2 - Experiments and Modeling

AU - Bahlmann, L. M.

AU - Smits, K. M.

AU - Heck, K.

AU - Coltman, E.

AU - Helmig, R.

AU - Neuweiler, I.

N1 - Funding Information: This work has been funded by the German Research Foundation (Deutsche Forschungsgemeinschaft [DFG]) under Projects NE 824/14‐1 and 327154368 and by the U.S. National Science Foundation under Project 1447533. We thank the DFG and the U.S. National Science Foundation for their support.

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N2 - We investigate the influence of near-surface wind conditions on subsurface gas transport and on soil-atmosphere gas exchange for gases of different density. Results of a sand tank experiment are supported by a numerical investigation with a fully coupled porous medium-free flow model, which accounts for wind turbulence. The experiment consists of a two-dimensional bench-scale soil tank containing homogeneous sand and an overlying wind tunnel. A point source was installed at the bottom of the tank. Gas concentrations were measured at multiple horizontal and vertical locations. Tested conditions include four wind velocities (0.2/1.0/2.0/2.7 m/s), three different gases (helium: light, nitrogen: neutral, and carbon dioxide: heavy), and two transport cases (1: steady-state gas supply from the point source; 2: transport under decreasing concentration gradient, subsequent to termination of gas supply). The model was used to assess flow patterns and gas fluxes across the soil surface. Results demonstrate that flow and transport in the vicinity of the surface are strongly coupled to the overlying wind field. An increase in wind velocity accelerates soil-atmosphere gas exchange. This is due to the effect of the wind profile on soil surface concentrations and due to wind-induced advection, which causes subsurface horizontal transport. The presence of gases with pronounced density difference to air adds additional complexity to the transport through the wind-affected soil layers. Wind impact differs between tested gases. Observed transport is multidimensional and shows that heavy as well as light gases cannot be treated as inert tracers, which applies to many gases in environmental studies.

AB - We investigate the influence of near-surface wind conditions on subsurface gas transport and on soil-atmosphere gas exchange for gases of different density. Results of a sand tank experiment are supported by a numerical investigation with a fully coupled porous medium-free flow model, which accounts for wind turbulence. The experiment consists of a two-dimensional bench-scale soil tank containing homogeneous sand and an overlying wind tunnel. A point source was installed at the bottom of the tank. Gas concentrations were measured at multiple horizontal and vertical locations. Tested conditions include four wind velocities (0.2/1.0/2.0/2.7 m/s), three different gases (helium: light, nitrogen: neutral, and carbon dioxide: heavy), and two transport cases (1: steady-state gas supply from the point source; 2: transport under decreasing concentration gradient, subsequent to termination of gas supply). The model was used to assess flow patterns and gas fluxes across the soil surface. Results demonstrate that flow and transport in the vicinity of the surface are strongly coupled to the overlying wind field. An increase in wind velocity accelerates soil-atmosphere gas exchange. This is due to the effect of the wind profile on soil surface concentrations and due to wind-induced advection, which causes subsurface horizontal transport. The presence of gases with pronounced density difference to air adds additional complexity to the transport through the wind-affected soil layers. Wind impact differs between tested gases. Observed transport is multidimensional and shows that heavy as well as light gases cannot be treated as inert tracers, which applies to many gases in environmental studies.

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