Effect of moisture on the nonlinear viscoelastic fracture behavior of polymer nanocompsites: a finite deformation phase-field model

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Original languageEnglish
Pages (from-to)773-790
Number of pages18
JournalEngineering with computers
Volume39
Issue number1
Early online date23 May 2022
Publication statusPublished - Feb 2023

Abstract

The mechanisms underlying damage in high-performance polymer nanocomposites are remarkably affected by hygrothermal conditions. In this study, we develop a phase-field formulation to investigate the influence of hygrothermal conditions on the nonlinear viscoelastic fracture behavior of epoxy resins and their nanocomposites at finite deformation. For this, the Helmholtz free energy, capturing the effect of temperature and moisture and nanoparticle contents, is defined based on an additive decomposition of the energy into an equilibrium, a non-equilibrium, and a volumetric contribution with different definitions under tensile and compressive loading. The coupled displacement phase-field problem is solved using a quasi-Newton monolithic algorithm and a staggered solution scheme. Numerical examples show that the monolithic algorithm is more efficient. Simulations are performed to investigate the effect of temperature, deformation rate, and moisture content on the force–displacement response of boehmite nanoparticle/epoxy samples in benchmark numerical problems. Comparing numerical predictions and experimental data for compact-tension tests shows good agreement at different nanoparticle contents. Also, the model’s capability to predict fracture patterns is evaluated using simulations of single-edge notched nanocomposite plates under tensile and shear loading.

Keywords

    Finite deformation, Finite element, Nanocomposite, Nonlinear viscoelasticity, Phase-field modeling

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Effect of moisture on the nonlinear viscoelastic fracture behavior of polymer nanocompsites: a finite deformation phase-field model. / Arash, Behrouz; Exner, Wibke; Rolfes, Raimund.
In: Engineering with computers, Vol. 39, No. 1, 02.2023, p. 773-790.

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abstract = "The mechanisms underlying damage in high-performance polymer nanocomposites are remarkably affected by hygrothermal conditions. In this study, we develop a phase-field formulation to investigate the influence of hygrothermal conditions on the nonlinear viscoelastic fracture behavior of epoxy resins and their nanocomposites at finite deformation. For this, the Helmholtz free energy, capturing the effect of temperature and moisture and nanoparticle contents, is defined based on an additive decomposition of the energy into an equilibrium, a non-equilibrium, and a volumetric contribution with different definitions under tensile and compressive loading. The coupled displacement phase-field problem is solved using a quasi-Newton monolithic algorithm and a staggered solution scheme. Numerical examples show that the monolithic algorithm is more efficient. Simulations are performed to investigate the effect of temperature, deformation rate, and moisture content on the force–displacement response of boehmite nanoparticle/epoxy samples in benchmark numerical problems. Comparing numerical predictions and experimental data for compact-tension tests shows good agreement at different nanoparticle contents. Also, the model{\textquoteright}s capability to predict fracture patterns is evaluated using simulations of single-edge notched nanocomposite plates under tensile and shear loading.",
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author = "Behrouz Arash and Wibke Exner and Raimund Rolfes",
note = "Funding Information: This work originates from “Challenges of industrial application of nanomodified and hybrid material systems in lightweight rotor blade construction”(“HANNAH - Herausforderungen der industriellen Anwendung von nanomodifizierten und hybriden Werkstoffsystemen im Rotorblattleichtbau”) research project funded by the Federal Ministry for Economic Affairs and Energy. The authors wish to express their gratitude for the financial support. The authors also acknowledge the support of the LUIS scientific computing cluster, which is funded by Leibniz Universit{\"a}t Hannover, the Lower Saxony Ministry of Science and Culture (MWK), and the German Research Council (DFG).",
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AU - Arash, Behrouz

AU - Exner, Wibke

AU - Rolfes, Raimund

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PY - 2023/2

Y1 - 2023/2

N2 - The mechanisms underlying damage in high-performance polymer nanocomposites are remarkably affected by hygrothermal conditions. In this study, we develop a phase-field formulation to investigate the influence of hygrothermal conditions on the nonlinear viscoelastic fracture behavior of epoxy resins and their nanocomposites at finite deformation. For this, the Helmholtz free energy, capturing the effect of temperature and moisture and nanoparticle contents, is defined based on an additive decomposition of the energy into an equilibrium, a non-equilibrium, and a volumetric contribution with different definitions under tensile and compressive loading. The coupled displacement phase-field problem is solved using a quasi-Newton monolithic algorithm and a staggered solution scheme. Numerical examples show that the monolithic algorithm is more efficient. Simulations are performed to investigate the effect of temperature, deformation rate, and moisture content on the force–displacement response of boehmite nanoparticle/epoxy samples in benchmark numerical problems. Comparing numerical predictions and experimental data for compact-tension tests shows good agreement at different nanoparticle contents. Also, the model’s capability to predict fracture patterns is evaluated using simulations of single-edge notched nanocomposite plates under tensile and shear loading.

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