Determination of ionization and tunneling times in high-order harmonic generation

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Original languageEnglish
Article number043901
JournalPhysical Review Letters
Volume111
Issue number4
Publication statusPublished - 26 Jul 2013

Abstract

From the numerical solution of the time-dependent Schrödinger equation, we obtain the times of ionization and return of the laser-driven electron in high-order harmonic generation by probing the dynamics with a second harmonic field polarized orthogonal to the fundamental field and observing the harmonic emission in dependence on the two-color delay. Our retrieval method using complex-time evolution gives ionization and return times in excellent agreement with the quantum-orbit model, while a retrieval based on real-time classical dynamics can introduce substantial errors. Because of the imaginary parts, the harmonic signal polarized along the probe field is nonzero for any two-color delay. The tunneling time can be retrieved under an assumption for the return time.

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Determination of ionization and tunneling times in high-order harmonic generation. / Zhao, Jing; Lein, Manfred.
In: Physical Review Letters, Vol. 111, No. 4, 043901, 26.07.2013.

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abstract = "From the numerical solution of the time-dependent Schr{\"o}dinger equation, we obtain the times of ionization and return of the laser-driven electron in high-order harmonic generation by probing the dynamics with a second harmonic field polarized orthogonal to the fundamental field and observing the harmonic emission in dependence on the two-color delay. Our retrieval method using complex-time evolution gives ionization and return times in excellent agreement with the quantum-orbit model, while a retrieval based on real-time classical dynamics can introduce substantial errors. Because of the imaginary parts, the harmonic signal polarized along the probe field is nonzero for any two-color delay. The tunneling time can be retrieved under an assumption for the return time.",
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