Controlling conductivity by quantum well states in ultrathin Bi(111) films

Research output: Contribution to journalArticleResearchpeer review

Authors

  • Philipp Kröger
  • D. Abdelbarey
  • Marianna Siemens
  • Daniel Lükermann
  • S. Sologub
  • Herbert Pfnür
  • Christoph Tegenkamp

External Research Organisations

  • Institute of Physics National Academy of Sciences in Ukraine
  • Chemnitz University of Technology (CUT)
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Details

Original languageEnglish
Article number045403
JournalPhysical Review B
Volume97
Issue number4
Publication statusPublished - 3 Jan 2018

Abstract

Epitaxial Bi(111) films were subject to many and partly even controversial studies on the semimetal-semiconductor transition triggered by a robust quantum confinement. The residual conductance was ascribed to conducting surface channels. We investigated ultrathin crystalline Bi films on Si(111) as a function of film thickness d between 20 and 100 bilayers by means of electric transport measurements. Varying temperature and magnetic field, we disentangled two transport channels. One remains indeed metallic at all thicknesses investigated and exhibits a slightly increasing conductance as a function of d, whereas the second is activated with a d-1 dependence of the activation energy, indicating a quasiharmonic confining potential. Both channels reflect the electronic properties of the entire film and do not allow us to strictly separate surface and bulk states. While there is clearly no bulk conductivity, the activated channel is consistently described as electronic excitation into the partly occupied quantum well states, which are also responsible for the metallic conductance and preferentially located close to both interfaces of the film.

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Cite this

Controlling conductivity by quantum well states in ultrathin Bi(111) films. / Kröger, Philipp; Abdelbarey, D.; Siemens, Marianna et al.
In: Physical Review B, Vol. 97, No. 4, 045403, 03.01.2018.

Research output: Contribution to journalArticleResearchpeer review

Kröger, P, Abdelbarey, D, Siemens, M, Lükermann, D, Sologub, S, Pfnür, H & Tegenkamp, C 2018, 'Controlling conductivity by quantum well states in ultrathin Bi(111) films', Physical Review B, vol. 97, no. 4, 045403. https://doi.org/10.1103/physrevb.97.045403
Kröger, P., Abdelbarey, D., Siemens, M., Lükermann, D., Sologub, S., Pfnür, H., & Tegenkamp, C. (2018). Controlling conductivity by quantum well states in ultrathin Bi(111) films. Physical Review B, 97(4), Article 045403. https://doi.org/10.1103/physrevb.97.045403
Kröger P, Abdelbarey D, Siemens M, Lükermann D, Sologub S, Pfnür H et al. Controlling conductivity by quantum well states in ultrathin Bi(111) films. Physical Review B. 2018 Jan 3;97(4):045403. doi: 10.1103/physrevb.97.045403
Kröger, Philipp ; Abdelbarey, D. ; Siemens, Marianna et al. / Controlling conductivity by quantum well states in ultrathin Bi(111) films. In: Physical Review B. 2018 ; Vol. 97, No. 4.
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abstract = "Epitaxial Bi(111) films were subject to many and partly even controversial studies on the semimetal-semiconductor transition triggered by a robust quantum confinement. The residual conductance was ascribed to conducting surface channels. We investigated ultrathin crystalline Bi films on Si(111) as a function of film thickness d between 20 and 100 bilayers by means of electric transport measurements. Varying temperature and magnetic field, we disentangled two transport channels. One remains indeed metallic at all thicknesses investigated and exhibits a slightly increasing conductance as a function of d, whereas the second is activated with a d-1 dependence of the activation energy, indicating a quasiharmonic confining potential. Both channels reflect the electronic properties of the entire film and do not allow us to strictly separate surface and bulk states. While there is clearly no bulk conductivity, the activated channel is consistently described as electronic excitation into the partly occupied quantum well states, which are also responsible for the metallic conductance and preferentially located close to both interfaces of the film.",
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AU - Pfnür, Herbert

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