Details
| Original language | English |
|---|---|
| Pages (from-to) | 3609-3614 |
| Number of pages | 6 |
| Journal | Journal of Chemical Physics |
| Volume | 113 |
| Issue number | 9 |
| Publication status | Published - 21 Aug 2000 |
| Externally published | Yes |
Abstract
This paper shows that it is, in principle, possible to construct complex-valued nuclear wave packets describing photofragments produced through short-pulse excitation. This requires the experimental determination of the fragment kinetic-energy distribution and a pump-probe signal detecting the products. These sets of data yield the wave-packet densities in momentum and coordinate space. The phases of the wave function can be obtained from an iteration scheme. By investigating several examples, this paper shows that the algorithm works excellent even in unfavorable cases.
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In: Journal of Chemical Physics, Vol. 113, No. 9, 21.08.2000, p. 3609-3614.
Research output: Contribution to journal › Article › Research › peer review
}
TY - JOUR
T1 - Characterization of nuclear wave packets describing molecular photodissociation
AU - Lein, Manfred
AU - Erdmann, Martin
AU - Engel, Volker
N1 - Copyright: Copyright 2018 Elsevier B.V., All rights reserved.
PY - 2000/8/21
Y1 - 2000/8/21
N2 - This paper shows that it is, in principle, possible to construct complex-valued nuclear wave packets describing photofragments produced through short-pulse excitation. This requires the experimental determination of the fragment kinetic-energy distribution and a pump-probe signal detecting the products. These sets of data yield the wave-packet densities in momentum and coordinate space. The phases of the wave function can be obtained from an iteration scheme. By investigating several examples, this paper shows that the algorithm works excellent even in unfavorable cases.
AB - This paper shows that it is, in principle, possible to construct complex-valued nuclear wave packets describing photofragments produced through short-pulse excitation. This requires the experimental determination of the fragment kinetic-energy distribution and a pump-probe signal detecting the products. These sets of data yield the wave-packet densities in momentum and coordinate space. The phases of the wave function can be obtained from an iteration scheme. By investigating several examples, this paper shows that the algorithm works excellent even in unfavorable cases.
UR - http://www.scopus.com/inward/record.url?scp=0034271104&partnerID=8YFLogxK
U2 - 10.1063/1.1287718
DO - 10.1063/1.1287718
M3 - Article
AN - SCOPUS:0034271104
VL - 113
SP - 3609
EP - 3614
JO - Journal of Chemical Physics
JF - Journal of Chemical Physics
SN - 0021-9606
IS - 9
ER -