Carrier relaxation and electronic structure in InAs self-assembled quantum dots

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  • University of California at Santa Barbara
  • Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU Erlangen-Nürnberg)
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Original languageEnglish
Pages (from-to)11346-11353
Number of pages8
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume54
Issue number16
Publication statusPublished - 15 Oct 1996
Externally publishedYes

Abstract

We studied the electronic structure and relaxation processes in InAs quantum dots embedded in GaAs. Using capacitance measurements along with photoluminescence spectroscopy, we estimate the energy splitting between the ground and first excited quantum-dot state in the conduction and valence band, respectively. There are five quantum-dot transitions observable in our photoluminescence (PL) spectra, which we attribute to allowed transitions between electron and hole states of the same quantum number. Phonon-related relaxation processes were studied combining PL, resonant PL (RPL), and photoluminescence excitation (PLE) experiments. In the RPL as well as in the PLE spectra, we observed enhanced signals at twice the phonon energies available in the system. Therefore, a maximum in the intensity of the PLE and RPL signal does not necessarily occur when most of the dots are pumped resonantly into an excited state. The main criterion, however, seems to be that the energy distance between the pumped levels and the levels below matches a multiple of the available phonon energies. Changing the pump power in our resonant PL experiments corroborates that at least in the small carrier density regime phonon-related processes are important for the carrier relaxation in InAs quantum dots embedded in GaAs bulk material.

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Carrier relaxation and electronic structure in InAs self-assembled quantum dots. / Schmidt, Klaus H.; Medeiros-Ribeiro, G.; Oestreich, Michael et al.
In: Physical Review B - Condensed Matter and Materials Physics, Vol. 54, No. 16, 15.10.1996, p. 11346-11353.

Research output: Contribution to journalArticleResearchpeer review

Schmidt KH, Medeiros-Ribeiro G, Oestreich M, Petroff P, Döhler G. Carrier relaxation and electronic structure in InAs self-assembled quantum dots. Physical Review B - Condensed Matter and Materials Physics. 1996 Oct 15;54(16):11346-11353. doi: 10.1103/PhysRevB.54.11346
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AU - Schmidt, Klaus H.

AU - Medeiros-Ribeiro, G.

AU - Oestreich, Michael

AU - Petroff, P.

AU - Döhler, G.

PY - 1996/10/15

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N2 - We studied the electronic structure and relaxation processes in InAs quantum dots embedded in GaAs. Using capacitance measurements along with photoluminescence spectroscopy, we estimate the energy splitting between the ground and first excited quantum-dot state in the conduction and valence band, respectively. There are five quantum-dot transitions observable in our photoluminescence (PL) spectra, which we attribute to allowed transitions between electron and hole states of the same quantum number. Phonon-related relaxation processes were studied combining PL, resonant PL (RPL), and photoluminescence excitation (PLE) experiments. In the RPL as well as in the PLE spectra, we observed enhanced signals at twice the phonon energies available in the system. Therefore, a maximum in the intensity of the PLE and RPL signal does not necessarily occur when most of the dots are pumped resonantly into an excited state. The main criterion, however, seems to be that the energy distance between the pumped levels and the levels below matches a multiple of the available phonon energies. Changing the pump power in our resonant PL experiments corroborates that at least in the small carrier density regime phonon-related processes are important for the carrier relaxation in InAs quantum dots embedded in GaAs bulk material.

AB - We studied the electronic structure and relaxation processes in InAs quantum dots embedded in GaAs. Using capacitance measurements along with photoluminescence spectroscopy, we estimate the energy splitting between the ground and first excited quantum-dot state in the conduction and valence band, respectively. There are five quantum-dot transitions observable in our photoluminescence (PL) spectra, which we attribute to allowed transitions between electron and hole states of the same quantum number. Phonon-related relaxation processes were studied combining PL, resonant PL (RPL), and photoluminescence excitation (PLE) experiments. In the RPL as well as in the PLE spectra, we observed enhanced signals at twice the phonon energies available in the system. Therefore, a maximum in the intensity of the PLE and RPL signal does not necessarily occur when most of the dots are pumped resonantly into an excited state. The main criterion, however, seems to be that the energy distance between the pumped levels and the levels below matches a multiple of the available phonon energies. Changing the pump power in our resonant PL experiments corroborates that at least in the small carrier density regime phonon-related processes are important for the carrier relaxation in InAs quantum dots embedded in GaAs bulk material.

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