Bright single-photon emission from a GeV center in diamond under a microfabricated solid immersion lens at room temperature

Research output: Contribution to journalArticleResearchpeer review

Authors

  • J. Christinck
  • F. Hirt
  • H. Hofer
  • Z. Liu
  • M. Etzkorn
  • T. Dunatov
  • M. Jakšić
  • J. Forneris
  • S. Kück

External Research Organisations

  • Physikalisch-Technische Bundesanstalt PTB
  • Technische Universität Braunschweig
  • Ruder Boskovic Institute
  • University of Turin
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Details

Original languageEnglish
Article number193102
JournalJournal of applied physics
Volume133
Issue number19
Early online date16 May 2023
Publication statusPublished - 21 May 2023
Externally publishedYes

Abstract

We report on the metrological characterization of the emission from a germanium-vacancy center in diamond under a microfabricated solid immersion lens in a confocal laser-scanning microscope setup. Ge ions were implanted into a synthetic diamond at 3 MeV, and germanium-vacancy centers were then formed by subsequent annealing. Afterward, solid immersion lenses were fabricated in a focused ion beam scanning electron microscope. The photoluminescence was investigated at room temperature in terms of the spectral distribution, the excited state lifetime, the second-order correlation function, and the saturation behavior, proving simultaneous high single-photon purity and high brightness. Two methods were exploited to minimize the residual multi-photon probability: spectral filtering and temporal filtering. According to these results, we assume that Raman scattered photons and emission from neighboring color centers play an important role in the residual multi-photon emission probability. The system efficiency of the single-photon source was investigated and found to be in accordance with the value calculated from all sources of loss in the setup. The branching ratio of the germanium-vacancy center for the decay into the ground state and into metastable state was calculated. The results enable the usage of the single-photon source in future quantum radiometric experiments.

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Cite this

Bright single-photon emission from a GeV center in diamond under a microfabricated solid immersion lens at room temperature. / Christinck, J.; Hirt, F.; Hofer, H. et al.
In: Journal of applied physics, Vol. 133, No. 19, 193102, 21.05.2023.

Research output: Contribution to journalArticleResearchpeer review

Christinck, J, Hirt, F, Hofer, H, Liu, Z, Etzkorn, M, Dunatov, T, Jakšić, M, Forneris, J & Kück, S 2023, 'Bright single-photon emission from a GeV center in diamond under a microfabricated solid immersion lens at room temperature', Journal of applied physics, vol. 133, no. 19, 193102. https://doi.org/10.1063/5.0150208
Christinck, J., Hirt, F., Hofer, H., Liu, Z., Etzkorn, M., Dunatov, T., Jakšić, M., Forneris, J., & Kück, S. (2023). Bright single-photon emission from a GeV center in diamond under a microfabricated solid immersion lens at room temperature. Journal of applied physics, 133(19), Article 193102. https://doi.org/10.1063/5.0150208
Christinck J, Hirt F, Hofer H, Liu Z, Etzkorn M, Dunatov T et al. Bright single-photon emission from a GeV center in diamond under a microfabricated solid immersion lens at room temperature. Journal of applied physics. 2023 May 21;133(19):193102. Epub 2023 May 16. doi: 10.1063/5.0150208
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title = "Bright single-photon emission from a GeV center in diamond under a microfabricated solid immersion lens at room temperature",
abstract = "We report on the metrological characterization of the emission from a germanium-vacancy center in diamond under a microfabricated solid immersion lens in a confocal laser-scanning microscope setup. Ge ions were implanted into a synthetic diamond at 3 MeV, and germanium-vacancy centers were then formed by subsequent annealing. Afterward, solid immersion lenses were fabricated in a focused ion beam scanning electron microscope. The photoluminescence was investigated at room temperature in terms of the spectral distribution, the excited state lifetime, the second-order correlation function, and the saturation behavior, proving simultaneous high single-photon purity and high brightness. Two methods were exploited to minimize the residual multi-photon probability: spectral filtering and temporal filtering. According to these results, we assume that Raman scattered photons and emission from neighboring color centers play an important role in the residual multi-photon emission probability. The system efficiency of the single-photon source was investigated and found to be in accordance with the value calculated from all sources of loss in the setup. The branching ratio of the germanium-vacancy center for the decay into the ground state and into metastable state was calculated. The results enable the usage of the single-photon source in future quantum radiometric experiments.",
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note = "Funding Information: This work was funded by Project Nos. EMPIR 20FUN05 SEQUME and EMPIR 20IND05 QADeT. These projects have received funding from the EMPIR programme co-financed by the Participating States and from the European Union{\textquoteright}s 2020 research and innovation programme. This work was also funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany{\textquoteright}s Excellence Strategy—EXC 2123 QuantumFrontiers, Project No. 390837967. We gratefully acknowledge DFG support under Grant No. INST 188/452-1 FUGG, the support of the Braunschweig International Graduate School of Metrology B-IGSM and the DFG Research Training Group 1952 Metrology for Complex Nanosystems. We acknowledge financial support from the European Regional Development Fund for the “Center of Excellence for Advanced Materials and Sensing Devices” (Grant No. KK.01.1.1.01.0001).",
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AU - Christinck, J.

AU - Hirt, F.

AU - Hofer, H.

AU - Liu, Z.

AU - Etzkorn, M.

AU - Dunatov, T.

AU - Jakšić, M.

AU - Forneris, J.

AU - Kück, S.

N1 - Funding Information: This work was funded by Project Nos. EMPIR 20FUN05 SEQUME and EMPIR 20IND05 QADeT. These projects have received funding from the EMPIR programme co-financed by the Participating States and from the European Union’s 2020 research and innovation programme. This work was also funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany’s Excellence Strategy—EXC 2123 QuantumFrontiers, Project No. 390837967. We gratefully acknowledge DFG support under Grant No. INST 188/452-1 FUGG, the support of the Braunschweig International Graduate School of Metrology B-IGSM and the DFG Research Training Group 1952 Metrology for Complex Nanosystems. We acknowledge financial support from the European Regional Development Fund for the “Center of Excellence for Advanced Materials and Sensing Devices” (Grant No. KK.01.1.1.01.0001).

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Y1 - 2023/5/21

N2 - We report on the metrological characterization of the emission from a germanium-vacancy center in diamond under a microfabricated solid immersion lens in a confocal laser-scanning microscope setup. Ge ions were implanted into a synthetic diamond at 3 MeV, and germanium-vacancy centers were then formed by subsequent annealing. Afterward, solid immersion lenses were fabricated in a focused ion beam scanning electron microscope. The photoluminescence was investigated at room temperature in terms of the spectral distribution, the excited state lifetime, the second-order correlation function, and the saturation behavior, proving simultaneous high single-photon purity and high brightness. Two methods were exploited to minimize the residual multi-photon probability: spectral filtering and temporal filtering. According to these results, we assume that Raman scattered photons and emission from neighboring color centers play an important role in the residual multi-photon emission probability. The system efficiency of the single-photon source was investigated and found to be in accordance with the value calculated from all sources of loss in the setup. The branching ratio of the germanium-vacancy center for the decay into the ground state and into metastable state was calculated. The results enable the usage of the single-photon source in future quantum radiometric experiments.

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