Details
| Original language | English |
|---|---|
| Pages (from-to) | 5779-5782 |
| Number of pages | 4 |
| Journal | Chemical communications |
| Volume | 56 |
| Issue number | 43 |
| Early online date | 15 Apr 2020 |
| Publication status | Published - 28 May 2020 |
Abstract
An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.
ASJC Scopus subject areas
- Chemical Engineering(all)
- Catalysis
- Materials Science(all)
- Electronic, Optical and Magnetic Materials
- Materials Science(all)
- Ceramics and Composites
- Chemistry(all)
- General Chemistry
- Materials Science(all)
- Surfaces, Coatings and Films
- Materials Science(all)
- Metals and Alloys
- Materials Science(all)
- Materials Chemistry
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In: Chemical communications, Vol. 56, No. 43, 28.05.2020, p. 5779-5782.
Research output: Contribution to journal › Article › Research › peer review
}
TY - JOUR
T1 - Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst
AU - Fang, Wei
AU - Du, Chengfeng
AU - Kuang, Min
AU - Chen, Mengxin
AU - Huang, Wenjing
AU - Ren, Hao
AU - Xu, Jianwei
AU - Feldhoff, Armin
AU - Yan, Qingyu
N1 - Funding Information: This work was financially supported by Singapore MOE AcRF Tier 1 Grant No. 2016-T1-002-065, Tier 2 under Grant No. 2017-T2-2-069 and 2018-T2-01-010, as well as Deutsche Forschungs-gemeinschaft (DFG, German Research Foundation) FE928/21-1. The authors acknowledge the Facility for Analysis, Characterization, Testing and Simulation (FACTS) of Nanyang Technological University, Singapore, for technical support. The authors are grateful to F. Steinbach for assistance with TEM measurements.
PY - 2020/5/28
Y1 - 2020/5/28
N2 - An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.
AB - An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.
UR - http://www.scopus.com/inward/record.url?scp=85085598970&partnerID=8YFLogxK
U2 - 10.1039/d0cc01759k
DO - 10.1039/d0cc01759k
M3 - Article
C2 - 32322861
AN - SCOPUS:85085598970
VL - 56
SP - 5779
EP - 5782
JO - Chemical communications
JF - Chemical communications
SN - 1359-7345
IS - 43
ER -