Details
| Original language | English |
|---|---|
| Pages (from-to) | 212-217 |
| Number of pages | 6 |
| Journal | Chemical physics letters |
| Volume | 389 |
| Issue number | 1-3 |
| Early online date | 9 Apr 2004 |
| Publication status | Published - 1 May 2004 |
Abstract
We present experimental evidence of the existence of defect-induced turbulence in the NO+NH3 reaction on Pt{100}. The method is based upon the system dynamics reconstruction using time delay coordinates, and assuming that a two-dimensional representation is enough to capture the relevant dynamic features of the system. Since the reconstruction method by delay coordinates preserves the topology of the phase space, defects should appear as singularities localized at the center of the phase portraits. We also constructed the radial distribution function P(r) in which defects appear as a nonvanishing minimum at the origin (r=0).
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In: Chemical physics letters, Vol. 389, No. 1-3, 01.05.2004, p. 212-217.
Research output: Contribution to journal › Article › Research › peer review
}
TY - JOUR
T1 - An analysis of turbulent states in the NH3 + NO reaction on Pt{1 0 0}
AU - Irurzun, I. M.
AU - Imbihl, R.
AU - Vicente, J. L.
AU - Mola, E. E.
N1 - Funding Information: This work was financially supported by the Consejo Nacional de Investigaciones Científicas y Técnicas, CONICET, Universidad Nacional de La Plata, UNLP, Fundación Antorchas of Argentina, and DAAD.
PY - 2004/5/1
Y1 - 2004/5/1
N2 - We present experimental evidence of the existence of defect-induced turbulence in the NO+NH3 reaction on Pt{100}. The method is based upon the system dynamics reconstruction using time delay coordinates, and assuming that a two-dimensional representation is enough to capture the relevant dynamic features of the system. Since the reconstruction method by delay coordinates preserves the topology of the phase space, defects should appear as singularities localized at the center of the phase portraits. We also constructed the radial distribution function P(r) in which defects appear as a nonvanishing minimum at the origin (r=0).
AB - We present experimental evidence of the existence of defect-induced turbulence in the NO+NH3 reaction on Pt{100}. The method is based upon the system dynamics reconstruction using time delay coordinates, and assuming that a two-dimensional representation is enough to capture the relevant dynamic features of the system. Since the reconstruction method by delay coordinates preserves the topology of the phase space, defects should appear as singularities localized at the center of the phase portraits. We also constructed the radial distribution function P(r) in which defects appear as a nonvanishing minimum at the origin (r=0).
UR - http://www.scopus.com/inward/record.url?scp=1942445247&partnerID=8YFLogxK
U2 - 10.1016/j.cplett.2004.03.070
DO - 10.1016/j.cplett.2004.03.070
M3 - Article
AN - SCOPUS:1942445247
VL - 389
SP - 212
EP - 217
JO - Chemical physics letters
JF - Chemical physics letters
SN - 0009-2614
IS - 1-3
ER -