2D Surface Passivation in Semi-transparent Perovskite Top Solar Cells with Engineered Bandgap for Tandem Photovoltaics

Research output: Chapter in book/report/conference proceedingConference contributionResearchpeer review

Authors

  • Saba Gharibzadeh
  • Ihteaz M. Hossain
  • Paul Fassl
  • Adrian Mertens
  • Soren Schafer
  • Michael Rienacker
  • Tobias Wietler
  • Robby Peibst
  • Bryce S. Richards
  • Ulrich W. Paetzold

External Research Organisations

  • Karlsruhe Institute of Technology (KIT)
  • Institute for Solar Energy Research (ISFH)
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Details

Original languageEnglish
Title of host publication2020 47th IEEE Photovoltaic Specialists Conference, PVSC 2020
PublisherInstitute of Electrical and Electronics Engineers Inc.
Pages1344-1345
Number of pages2
ISBN (electronic)9781728161150
ISBN (print)978-1-7281-6116-7
Publication statusPublished - 2020
Event47th IEEE Photovoltaic Specialists Conference, PVSC 2020 - Calgary, Canada
Duration: 15 Jun 202021 Aug 2020

Publication series

NameConference Record of the IEEE Photovoltaic Specialists Conference
Volume2020-June
ISSN (Print)0160-8371

Abstract

Wide-bandgap perovskite top solar cells (PSCs) with optimal bandgap (Eg) are key to boost the efficiency of perovskite/Si tandem devices beyond the Shockley-Queisser limit for single-junction solar cells. However, the large open circuit voltage (Voc) deficit in the optimal bandgap range and the poor transmission of the top semi-transparent perovskite solar cells (s-PSCs) restricts the development in this field. Here, we present a novel 2D/3D perovskite heterostructure architecture to reduce the voltage deficit in PSCs. The reduced voltage deficit is a result of the decreased non-radiative recombination losses at the perovskite/hole-transport layer interface. Employing the 2D/3D perovskite heterostructure, efficient four-terminal (4T) perovskite/Si tandem solar cells with a stabilized power conversion efficiency (PCE) of up to 25.7% is demonstrated. In order to improve the PCE further, we present alternative transparent conductive oxide electrodes that reduce the parasitic absorption and reflection losses and enhances the transmission in the near infrared wavelengths, leading to a potential PCE of 27.4% for 4T perovskite/c-Si tandem devices.

Keywords

    2D/3D heterostructure, passivation layer, perovskite, poly-Si, silicon, tandem solar cells, wide-bandgap

ASJC Scopus subject areas

Cite this

2D Surface Passivation in Semi-transparent Perovskite Top Solar Cells with Engineered Bandgap for Tandem Photovoltaics. / Gharibzadeh, Saba; Hossain, Ihteaz M.; Fassl, Paul et al.
2020 47th IEEE Photovoltaic Specialists Conference, PVSC 2020. Institute of Electrical and Electronics Engineers Inc., 2020. p. 1344-1345 9300952 (Conference Record of the IEEE Photovoltaic Specialists Conference; Vol. 2020-June).

Research output: Chapter in book/report/conference proceedingConference contributionResearchpeer review

Gharibzadeh, S, Hossain, IM, Fassl, P, Mertens, A, Schafer, S, Rienacker, M, Wietler, T, Peibst, R, Richards, BS & Paetzold, UW 2020, 2D Surface Passivation in Semi-transparent Perovskite Top Solar Cells with Engineered Bandgap for Tandem Photovoltaics. in 2020 47th IEEE Photovoltaic Specialists Conference, PVSC 2020., 9300952, Conference Record of the IEEE Photovoltaic Specialists Conference, vol. 2020-June, Institute of Electrical and Electronics Engineers Inc., pp. 1344-1345, 47th IEEE Photovoltaic Specialists Conference, PVSC 2020, Calgary, Canada, 15 Jun 2020. https://doi.org/10.1109/PVSC45281.2020.9300952
Gharibzadeh, S., Hossain, I. M., Fassl, P., Mertens, A., Schafer, S., Rienacker, M., Wietler, T., Peibst, R., Richards, B. S., & Paetzold, U. W. (2020). 2D Surface Passivation in Semi-transparent Perovskite Top Solar Cells with Engineered Bandgap for Tandem Photovoltaics. In 2020 47th IEEE Photovoltaic Specialists Conference, PVSC 2020 (pp. 1344-1345). Article 9300952 (Conference Record of the IEEE Photovoltaic Specialists Conference; Vol. 2020-June). Institute of Electrical and Electronics Engineers Inc.. https://doi.org/10.1109/PVSC45281.2020.9300952
Gharibzadeh S, Hossain IM, Fassl P, Mertens A, Schafer S, Rienacker M et al. 2D Surface Passivation in Semi-transparent Perovskite Top Solar Cells with Engineered Bandgap for Tandem Photovoltaics. In 2020 47th IEEE Photovoltaic Specialists Conference, PVSC 2020. Institute of Electrical and Electronics Engineers Inc. 2020. p. 1344-1345. 9300952. (Conference Record of the IEEE Photovoltaic Specialists Conference). doi: 10.1109/PVSC45281.2020.9300952
Gharibzadeh, Saba ; Hossain, Ihteaz M. ; Fassl, Paul et al. / 2D Surface Passivation in Semi-transparent Perovskite Top Solar Cells with Engineered Bandgap for Tandem Photovoltaics. 2020 47th IEEE Photovoltaic Specialists Conference, PVSC 2020. Institute of Electrical and Electronics Engineers Inc., 2020. pp. 1344-1345 (Conference Record of the IEEE Photovoltaic Specialists Conference).
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AU - Gharibzadeh, Saba

AU - Hossain, Ihteaz M.

AU - Fassl, Paul

AU - Mertens, Adrian

AU - Schafer, Soren

AU - Rienacker, Michael

AU - Wietler, Tobias

AU - Peibst, Robby

AU - Richards, Bryce S.

AU - Paetzold, Ulrich W.

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