The role of thermal and electronic pressure in the picosecond acoustic response of femtosecond laser-excited solids

Publikation: Beitrag in Buch/Bericht/Sammelwerk/KonferenzbandAufsatz in KonferenzbandForschungPeer-Review

Autoren

  • Uladzimir Shymanovich
  • Matthieu Nicoul
  • Stefan Kähle
  • Wei Lu
  • Alexander Tarasevitch
  • Ping Zhou
  • Tobias Wietler
  • Michael Horn Von Hoegen
  • Dietrich Von Der Linde
  • Klaus Sokolowski-Tinten

Externe Organisationen

  • Universität Duisburg-Essen
  • Universität zu Köln
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Details

OriginalspracheEnglisch
Titel des SammelwerksUltrafast Processes in Materials Science
Seiten111-116
Seitenumfang6
PublikationsstatusVeröffentlicht - 2010
Veranstaltung2009 MRS Fall Meeting - Boston, USA / Vereinigte Staaten
Dauer: 30 Nov. 20094 Dez. 2009

Publikationsreihe

NameMaterials Research Society Symposium Proceedings
Band1230
ISSN (Print)0272-9172

Abstract

In this work we apply ultrafast time-resolved X-ray diffraction to study the dynamics of coherent acoustic phonons in laser-excited Ge and Au, with the particular goal to clarify the interplay of the electronic and thermal driving forces. For Ge our measurements reveal that the relative strength of the electronic pressure decreases with increasing laser fluence. For larger laser fluences the thermal pressure exceeds the electronic one, and only at low excitation strength the electronic pressure becomes the dominant driving force, as predicted by theory [1]. For the case of Au the data are well described within the established theoretical framework using the known values for those material parameters which determine the laser-induced pressure, namely the energy relaxation time and the electronic and lattice Grüneisen parameters.

ASJC Scopus Sachgebiete

Zitieren

The role of thermal and electronic pressure in the picosecond acoustic response of femtosecond laser-excited solids. / Shymanovich, Uladzimir; Nicoul, Matthieu; Kähle, Stefan et al.
Ultrafast Processes in Materials Science. 2010. S. 111-116 (Materials Research Society Symposium Proceedings; Band 1230).

Publikation: Beitrag in Buch/Bericht/Sammelwerk/KonferenzbandAufsatz in KonferenzbandForschungPeer-Review

Shymanovich, U, Nicoul, M, Kähle, S, Lu, W, Tarasevitch, A, Zhou, P, Wietler, T, Von Hoegen, MH, Von Der Linde, D & Sokolowski-Tinten, K 2010, The role of thermal and electronic pressure in the picosecond acoustic response of femtosecond laser-excited solids. in Ultrafast Processes in Materials Science. Materials Research Society Symposium Proceedings, Bd. 1230, S. 111-116, 2009 MRS Fall Meeting, Boston, Massachusetts, USA / Vereinigte Staaten, 30 Nov. 2009.
Shymanovich, U., Nicoul, M., Kähle, S., Lu, W., Tarasevitch, A., Zhou, P., Wietler, T., Von Hoegen, M. H., Von Der Linde, D., & Sokolowski-Tinten, K. (2010). The role of thermal and electronic pressure in the picosecond acoustic response of femtosecond laser-excited solids. In Ultrafast Processes in Materials Science (S. 111-116). (Materials Research Society Symposium Proceedings; Band 1230).
Shymanovich U, Nicoul M, Kähle S, Lu W, Tarasevitch A, Zhou P et al. The role of thermal and electronic pressure in the picosecond acoustic response of femtosecond laser-excited solids. in Ultrafast Processes in Materials Science. 2010. S. 111-116. (Materials Research Society Symposium Proceedings).
Shymanovich, Uladzimir ; Nicoul, Matthieu ; Kähle, Stefan et al. / The role of thermal and electronic pressure in the picosecond acoustic response of femtosecond laser-excited solids. Ultrafast Processes in Materials Science. 2010. S. 111-116 (Materials Research Society Symposium Proceedings).
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abstract = "In this work we apply ultrafast time-resolved X-ray diffraction to study the dynamics of coherent acoustic phonons in laser-excited Ge and Au, with the particular goal to clarify the interplay of the electronic and thermal driving forces. For Ge our measurements reveal that the relative strength of the electronic pressure decreases with increasing laser fluence. For larger laser fluences the thermal pressure exceeds the electronic one, and only at low excitation strength the electronic pressure becomes the dominant driving force, as predicted by theory [1]. For the case of Au the data are well described within the established theoretical framework using the known values for those material parameters which determine the laser-induced pressure, namely the energy relaxation time and the electronic and lattice Gr{\"u}neisen parameters.",
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AU - Shymanovich, Uladzimir

AU - Nicoul, Matthieu

AU - Kähle, Stefan

AU - Lu, Wei

AU - Tarasevitch, Alexander

AU - Zhou, Ping

AU - Wietler, Tobias

AU - Von Hoegen, Michael Horn

AU - Von Der Linde, Dietrich

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