Details
| Originalsprache | Englisch |
|---|---|
| Aufsatznummer | e023412 |
| Fachzeitschrift | Physical Review A |
| Jahrgang | 93 |
| Ausgabenummer | 2 |
| Publikationsstatus | Veröffentlicht - 11 Feb. 2016 |
Abstract
Strong-field ionization (SFI) has been shown to prepare wave packets with few-femtosecond periods. Here, we explore whether this technique can be extended to the attosecond time scale. We introduce an intuitive model, which is based on the Fourier transform of the subcycle SFI rate, for predicting the bandwidth of ionic states that can be coherently prepared by SFI. The coherent bandwidth decreases considerably with increasing central wavelength of the ionizing pulse but it is much less sensitive to its intensity. Many-body calculations based on time-dependent configuration-interaction singles support these results. The influence of channel interactions and laser-induced dynamics within the ion is discussed. Our results further predict that multicycle femtosecond pulses can coherently prepare subfemtosecond wave packets with higher selectivity and versatility compared to single-cycle pulses with an additional sensitivity to the mutual parity of the prepared states.
ASJC Scopus Sachgebiete
- Physik und Astronomie (insg.)
- Atom- und Molekularphysik sowie Optik
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in: Physical Review A, Jahrgang 93, Nr. 2, e023412, 11.02.2016.
Publikation: Beitrag in Fachzeitschrift › Artikel › Forschung › Peer-Review
}
TY - JOUR
T1 - Preparing attosecond coherences by strong-field ionization
AU - Pabst, Stefan
AU - Lein, Manfred
AU - Wörner, Hans Jakob
PY - 2016/2/11
Y1 - 2016/2/11
N2 - Strong-field ionization (SFI) has been shown to prepare wave packets with few-femtosecond periods. Here, we explore whether this technique can be extended to the attosecond time scale. We introduce an intuitive model, which is based on the Fourier transform of the subcycle SFI rate, for predicting the bandwidth of ionic states that can be coherently prepared by SFI. The coherent bandwidth decreases considerably with increasing central wavelength of the ionizing pulse but it is much less sensitive to its intensity. Many-body calculations based on time-dependent configuration-interaction singles support these results. The influence of channel interactions and laser-induced dynamics within the ion is discussed. Our results further predict that multicycle femtosecond pulses can coherently prepare subfemtosecond wave packets with higher selectivity and versatility compared to single-cycle pulses with an additional sensitivity to the mutual parity of the prepared states.
AB - Strong-field ionization (SFI) has been shown to prepare wave packets with few-femtosecond periods. Here, we explore whether this technique can be extended to the attosecond time scale. We introduce an intuitive model, which is based on the Fourier transform of the subcycle SFI rate, for predicting the bandwidth of ionic states that can be coherently prepared by SFI. The coherent bandwidth decreases considerably with increasing central wavelength of the ionizing pulse but it is much less sensitive to its intensity. Many-body calculations based on time-dependent configuration-interaction singles support these results. The influence of channel interactions and laser-induced dynamics within the ion is discussed. Our results further predict that multicycle femtosecond pulses can coherently prepare subfemtosecond wave packets with higher selectivity and versatility compared to single-cycle pulses with an additional sensitivity to the mutual parity of the prepared states.
UR - http://www.scopus.com/inward/record.url?scp=84957991078&partnerID=8YFLogxK
U2 - 10.1103/PhysRevA.93.023412
DO - 10.1103/PhysRevA.93.023412
M3 - Article
AN - SCOPUS:84957991078
VL - 93
JO - Physical Review A
JF - Physical Review A
SN - 2469-9926
IS - 2
M1 - e023412
ER -