Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products

Publikation: Beitrag in Fachzeitschrift › Übersichtsarbeit › Forschung › Peer-Review

Autoren

  • Yongqian Cui
  • Abdelkader Labidi
  • Xinxin Liang
  • Xin Huang
  • Jingyi Wang
  • Ximing Li
  • Qibing Dong
  • Xiaolong Zhang
  • Sarah I. Othman
  • Ahmed A. Allam
  • Detlef W. Bahnemann
  • Chuanyi Wang

Organisationseinheiten

Externe Organisationen

  • Shaanxi University of Science and Technology
  • Princess Nourah bint Abdulrahman University
  • Al-Imam Muhammad Ibn Saud Islamic University
  • Staatliche Universität Sankt Petersburg
Forschungs-netzwerk anzeigen

Details

OriginalspracheEnglisch
Aufsatznummere202400551
FachzeitschriftCHEMSUSCHEM
Jahrgang17
Ausgabenummer18
Frühes Online-Datum15 Apr. 2024
PublikationsstatusVeröffentlicht - 24 Sept. 2024

Abstract

Over the past decades, CO2 greenhouse emission has been considerably increased, causing global warming and climate change. Indeed, converting CO2 into valuable chemicals and fuels is a desired option to resolve issues caused by its continuous emission into the atmosphere. Nevertheless, CO2 conversion has been hampered by the ultrahigh dissociation energy of C=O bonds, which makes it thermodynamically and kinetically challenging. From this prospect, photocatalytic approaches appear promising for CO2 reduction in terms of their efficiency compared to other traditional technologies. Thus, many efforts have been made in the designing of photocatalysts with asymmetric sites and oxygen vacancies, which can break the charge distribution balance of CO2 molecule, reduce hydrogenation energy barrier and accelerate CO2 conversion into chemicals and fuels. Here, we review the recent advances in CO2 hydrogenation to C1 and C2 products utilizing photocatalysis processes. We also pin down the key factors or parameters influencing the generation of C2 products during CO2 hydrogenation. In addition, the current status of CO2 reduction is summarized, projecting the future direction for CO2 conversion by photocatalysis processes.

ASJC Scopus Sachgebiete

Ziele für nachhaltige Entwicklung

Zitieren

Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products. / Cui, Yongqian; Labidi, Abdelkader; Liang, Xinxin et al.
in: CHEMSUSCHEM, Jahrgang 17, Nr. 18, e202400551, 24.09.2024.

Publikation: Beitrag in Fachzeitschrift › Übersichtsarbeit › Forschung › Peer-Review

Cui, Y, Labidi, A, Liang, X, Huang, X, Wang, J, Li, X, Dong, Q, Zhang, X, Othman, SI, Allam, AA, Bahnemann, DW & Wang, C 2024, 'Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products', CHEMSUSCHEM, Jg. 17, Nr. 18, e202400551. https://doi.org/10.1002/cssc.202400551
Cui, Y., Labidi, A., Liang, X., Huang, X., Wang, J., Li, X., Dong, Q., Zhang, X., Othman, S. I., Allam, A. A., Bahnemann, D. W., & Wang, C. (2024). Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products. CHEMSUSCHEM, 17(18), Artikel e202400551. https://doi.org/10.1002/cssc.202400551
Cui Y, Labidi A, Liang X, Huang X, Wang J, Li X et al. Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products. CHEMSUSCHEM. 2024 Sep 24;17(18):e202400551. Epub 2024 Apr 15. doi: 10.1002/cssc.202400551
Cui, Yongqian ; Labidi, Abdelkader ; Liang, Xinxin et al. / Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products. in: CHEMSUSCHEM. 2024 ; Jahrgang 17, Nr. 18.
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abstract = "Over the past decades, CO2 greenhouse emission has been considerably increased, causing global warming and climate change. Indeed, converting CO2 into valuable chemicals and fuels is a desired option to resolve issues caused by its continuous emission into the atmosphere. Nevertheless, CO2 conversion has been hampered by the ultrahigh dissociation energy of C=O bonds, which makes it thermodynamically and kinetically challenging. From this prospect, photocatalytic approaches appear promising for CO2 reduction in terms of their efficiency compared to other traditional technologies. Thus, many efforts have been made in the designing of photocatalysts with asymmetric sites and oxygen vacancies, which can break the charge distribution balance of CO2 molecule, reduce hydrogenation energy barrier and accelerate CO2 conversion into chemicals and fuels. Here, we review the recent advances in CO2 hydrogenation to C1 and C2 products utilizing photocatalysis processes. We also pin down the key factors or parameters influencing the generation of C2 products during CO2 hydrogenation. In addition, the current status of CO2 reduction is summarized, projecting the future direction for CO2 conversion by photocatalysis processes.",
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T1 - Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products

AU - Cui, Yongqian

AU - Labidi, Abdelkader

AU - Liang, Xinxin

AU - Huang, Xin

AU - Wang, Jingyi

AU - Li, Ximing

AU - Dong, Qibing

AU - Zhang, Xiaolong

AU - Othman, Sarah I.

AU - Allam, Ahmed A.

AU - Bahnemann, Detlef W.

AU - Wang, Chuanyi

N1 - Publisher Copyright: © 2024 Wiley-VCH GmbH.

PY - 2024/9/24

Y1 - 2024/9/24

N2 - Over the past decades, CO2 greenhouse emission has been considerably increased, causing global warming and climate change. Indeed, converting CO2 into valuable chemicals and fuels is a desired option to resolve issues caused by its continuous emission into the atmosphere. Nevertheless, CO2 conversion has been hampered by the ultrahigh dissociation energy of C=O bonds, which makes it thermodynamically and kinetically challenging. From this prospect, photocatalytic approaches appear promising for CO2 reduction in terms of their efficiency compared to other traditional technologies. Thus, many efforts have been made in the designing of photocatalysts with asymmetric sites and oxygen vacancies, which can break the charge distribution balance of CO2 molecule, reduce hydrogenation energy barrier and accelerate CO2 conversion into chemicals and fuels. Here, we review the recent advances in CO2 hydrogenation to C1 and C2 products utilizing photocatalysis processes. We also pin down the key factors or parameters influencing the generation of C2 products during CO2 hydrogenation. In addition, the current status of CO2 reduction is summarized, projecting the future direction for CO2 conversion by photocatalysis processes.

AB - Over the past decades, CO2 greenhouse emission has been considerably increased, causing global warming and climate change. Indeed, converting CO2 into valuable chemicals and fuels is a desired option to resolve issues caused by its continuous emission into the atmosphere. Nevertheless, CO2 conversion has been hampered by the ultrahigh dissociation energy of C=O bonds, which makes it thermodynamically and kinetically challenging. From this prospect, photocatalytic approaches appear promising for CO2 reduction in terms of their efficiency compared to other traditional technologies. Thus, many efforts have been made in the designing of photocatalysts with asymmetric sites and oxygen vacancies, which can break the charge distribution balance of CO2 molecule, reduce hydrogenation energy barrier and accelerate CO2 conversion into chemicals and fuels. Here, we review the recent advances in CO2 hydrogenation to C1 and C2 products utilizing photocatalysis processes. We also pin down the key factors or parameters influencing the generation of C2 products during CO2 hydrogenation. In addition, the current status of CO2 reduction is summarized, projecting the future direction for CO2 conversion by photocatalysis processes.

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