Multiple-collision induced dissociation of trapped silver clusters Agn+ (2≤n≤25)

Publikation: Beitrag in Fachzeitschrift › Artikel › Forschung › Peer-Review

Autorschaft

  • S. Krückeberg
  • G. Dietrich
  • K. Lützenkirchen
  • L. Schweikhard
  • Clemens Walther
  • J. Ziegler

Externe Organisationen

  • Johannes Gutenberg-Universität Mainz
  • Harvard University
  • SerCon GmbH
  • Institut de Recherches Subatomiques
  • Deutsche Bank AG
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Details

OriginalspracheEnglisch
Seiten (von - bis)7216-7227
Seitenumfang12
FachzeitschriftJournal of Chemical Physics
Jahrgang110
Ausgabenummer15
PublikationsstatusVeröffentlicht - 7 Apr. 1999
Extern publiziertJa

Abstract

The dissociation energies of singly charged silver cluster cations, Agn+ (2≤n≤25), are determined by multiple-collision induced dissociation (MCID) in a Penning trap. The fragment yield is analyzed in terms of a linearized impulsive collision theory for the energy transfer in the multicollisional process and the delayed decay as predicted by the Rice-Ramsperger-Kassel (RRK) model. Previous photofragmentation experiments performed in the size range (9≤n≤21) are found to be in good agreement with the present results. Theoretical predictions agree for most clusters sizes.

ASJC Scopus Sachgebiete

Zitieren

Multiple-collision induced dissociation of trapped silver clusters Agn+ (2≤n≤25). / Krückeberg, S.; Dietrich, G.; Lützenkirchen, K. et al.
in: Journal of Chemical Physics, Jahrgang 110, Nr. 15, 07.04.1999, S. 7216-7227.

Publikation: Beitrag in Fachzeitschrift › Artikel › Forschung › Peer-Review

Krückeberg, S, Dietrich, G, Lützenkirchen, K, Schweikhard, L, Walther, C & Ziegler, J 1999, 'Multiple-collision induced dissociation of trapped silver clusters Agn+ (2≤n≤25)', Journal of Chemical Physics, Jg. 110, Nr. 15, S. 7216-7227. https://doi.org/10.1063/1.478625
Krückeberg, S., Dietrich, G., Lützenkirchen, K., Schweikhard, L., Walther, C., & Ziegler, J. (1999). Multiple-collision induced dissociation of trapped silver clusters Agn+ (2≤n≤25). Journal of Chemical Physics, 110(15), 7216-7227. https://doi.org/10.1063/1.478625
Krückeberg S, Dietrich G, Lützenkirchen K, Schweikhard L, Walther C, Ziegler J. Multiple-collision induced dissociation of trapped silver clusters Agn+ (2≤n≤25). Journal of Chemical Physics. 1999 Apr 7;110(15):7216-7227. doi: 10.1063/1.478625
Krückeberg, S. ; Dietrich, G. ; Lützenkirchen, K. et al. / Multiple-collision induced dissociation of trapped silver clusters Agn+ (2≤n≤25). in: Journal of Chemical Physics. 1999 ; Jahrgang 110, Nr. 15. S. 7216-7227.
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T1 - Multiple-collision induced dissociation of trapped silver clusters Agn+ (2≤n≤25)

AU - Krückeberg, S.

AU - Dietrich, G.

AU - Lützenkirchen, K.

AU - Schweikhard, L.

AU - Walther, Clemens

AU - Ziegler, J.

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AB - The dissociation energies of singly charged silver cluster cations, Agn+ (2≤n≤25), are determined by multiple-collision induced dissociation (MCID) in a Penning trap. The fragment yield is analyzed in terms of a linearized impulsive collision theory for the energy transfer in the multicollisional process and the delayed decay as predicted by the Rice-Ramsperger-Kassel (RRK) model. Previous photofragmentation experiments performed in the size range (9≤n≤21) are found to be in good agreement with the present results. Theoretical predictions agree for most clusters sizes.

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