Details
| Titel in Übersetzung | Hoch fluoreszierende Pyridiniumbetaine für die Lichtsammlung |
|---|---|
| Originalsprache | Englisch |
| Seiten (von - bis) | 13882-13886 |
| Seitenumfang | 5 |
| Fachzeitschrift | Angewandte Chemie International Edition |
| Jahrgang | 56 |
| Ausgabenummer | 44 |
| Frühes Online-Datum | 10 Juli 2017 |
| Publikationsstatus | Veröffentlicht - 23 Okt. 2017 |
| Extern publiziert | Ja |
Abstract
We report the findings of our experimental and theoretical investigations into the properties of pyridinium enolates and their potential utility in light-harvesting applications, such as in luminescent solar concentrators (LSCs). We present the synthesis, structures, photophysical characterization, and wavefunction-based quantum-chemical studies of five cyclobetaines. The performance of an LSC device incorporating one of these cyclobetaines is shown to be comparable to state-of-the-art devices.
ASJC Scopus Sachgebiete
- Chemie (insg.)
- Allgemeine Chemie
- Chemische Verfahrenstechnik (insg.)
- Katalyse
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in: Angewandte Chemie International Edition, Jahrgang 56, Nr. 44, 23.10.2017, S. 13882-13886.
Publikation: Beitrag in Fachzeitschrift › Artikel › Forschung › Peer-Review
}
TY - JOUR
T1 - Highly Fluorescent Pyridinium Betaines for Light Harvesting
AU - Xu, Jingjing
AU - Zhang, Bolong
AU - Jansen, Marina
AU - Goerigk, Lars
AU - Wong, Wallace W. H.
AU - Ritchie, Chris
N1 - Funding information: This work was made possible by support from the Australian Renewable Energy Agency (ARENA), which funds the project grants within the Australian Centre for Advanced Photovoltaics. We thank the ARC for financial support through the grants DE140100550 (to L.G.), CE170100026 and FT130100500 (to W.W.H.W.), and DE130100615 (to C.R.). L.G. also thanks The University of Melbourne for additional financial support (RGSS2016), and the NCI and VLSCI for computing time. Responsibility for the views, information, or advice expressed herein is not accepted by the Australian Government.
PY - 2017/10/23
Y1 - 2017/10/23
N2 - We report the findings of our experimental and theoretical investigations into the properties of pyridinium enolates and their potential utility in light-harvesting applications, such as in luminescent solar concentrators (LSCs). We present the synthesis, structures, photophysical characterization, and wavefunction-based quantum-chemical studies of five cyclobetaines. The performance of an LSC device incorporating one of these cyclobetaines is shown to be comparable to state-of-the-art devices.
AB - We report the findings of our experimental and theoretical investigations into the properties of pyridinium enolates and their potential utility in light-harvesting applications, such as in luminescent solar concentrators (LSCs). We present the synthesis, structures, photophysical characterization, and wavefunction-based quantum-chemical studies of five cyclobetaines. The performance of an LSC device incorporating one of these cyclobetaines is shown to be comparable to state-of-the-art devices.
KW - betaines
KW - energy transfer
KW - fluorophores
KW - luminescent solar concentrators
UR - http://www.scopus.com/inward/record.url?scp=85031738033&partnerID=8YFLogxK
U2 - 10.1002/ange.201704832
DO - 10.1002/ange.201704832
M3 - Article
VL - 56
SP - 13882
EP - 13886
JO - Angewandte Chemie International Edition
JF - Angewandte Chemie International Edition
SN - 1433-7851
IS - 44
ER -