Femtosecond laser induced step-like structures inside transparent hydrogel due to laser induced threshold reduction

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Autoren

  • Emanuel Saerchen
  • Susann Liedtke-Gruener
  • Maximilian Kopp
  • Alexander Heisterkamp
  • Holger Lubatschowski
  • Tammo Ripken

Organisationseinheiten

Externe Organisationen

  • Laser Zentrum Hannover e.V. (LZH)
  • Rowiak GmbH
Forschungs-netzwerk anzeigen

Details

OriginalspracheEnglisch
Aufsatznummere0222293
FachzeitschriftPLOS ONE
Jahrgang14
Ausgabenummer9
Frühes Online-Datum1 Sept. 2019
PublikationsstatusElektronisch veröffentlicht (E-Pub) - 1 Sept. 2019

Abstract

In the area of laser material processing, versatile applications for cutting glasses and transparent polymers exist. However, parasitic effects such as the creation of step-like structures appear when laser cutting inside a transparent material. To date, these structures were only described empirically. This work establishes the physical and chemical mechanisms behind the observed effects and describes the influence of process and material parameters onto the creation of step-like structures in hydrogel, Dihydroxyethylmethacrylat (HEMA). By focusing laser pulses in HEMA, reduced pulse separation distance below 50 nm and rise in pulse energy enhances the creation of unintended step-like structures. Spatial resolved Raman-spectroscopy was used to measure the laser induced chemical modification, which results into a reduced breakdown threshold. The reduction in threshold influences the position of optical breakdown for the succeeding laser pulses and consequently leads to the step-like structures. Additionally, the experimental findings were supplemented with numerical simulations of the influence of reduced damage threshold onto the position of optical breakdown. In summary, chemical material change was defined as cause of the step-like structures. Furthermore, the parameters to avoid these structures were identified.

ASJC Scopus Sachgebiete

Zitieren

Femtosecond laser induced step-like structures inside transparent hydrogel due to laser induced threshold reduction. / Saerchen, Emanuel; Liedtke-Gruener, Susann; Kopp, Maximilian et al.
in: PLOS ONE, Jahrgang 14, Nr. 9, e0222293, 01.09.2019.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Saerchen, E., Liedtke-Gruener, S., Kopp, M., Heisterkamp, A., Lubatschowski, H., & Ripken, T. (2019). Femtosecond laser induced step-like structures inside transparent hydrogel due to laser induced threshold reduction. PLOS ONE, 14(9), Artikel e0222293. Vorabveröffentlichung online. https://doi.org/10.1371/journal.pone.0222293, https://doi.org/10.15488/10444
Saerchen E, Liedtke-Gruener S, Kopp M, Heisterkamp A, Lubatschowski H, Ripken T. Femtosecond laser induced step-like structures inside transparent hydrogel due to laser induced threshold reduction. PLOS ONE. 2019 Sep 1;14(9):e0222293. Epub 2019 Sep 1. doi: 10.1371/journal.pone.0222293, 10.15488/10444
Saerchen, Emanuel ; Liedtke-Gruener, Susann ; Kopp, Maximilian et al. / Femtosecond laser induced step-like structures inside transparent hydrogel due to laser induced threshold reduction. in: PLOS ONE. 2019 ; Jahrgang 14, Nr. 9.
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abstract = "In the area of laser material processing, versatile applications for cutting glasses and transparent polymers exist. However, parasitic effects such as the creation of step-like structures appear when laser cutting inside a transparent material. To date, these structures were only described empirically. This work establishes the physical and chemical mechanisms behind the observed effects and describes the influence of process and material parameters onto the creation of step-like structures in hydrogel, Dihydroxyethylmethacrylat (HEMA). By focusing laser pulses in HEMA, reduced pulse separation distance below 50 nm and rise in pulse energy enhances the creation of unintended step-like structures. Spatial resolved Raman-spectroscopy was used to measure the laser induced chemical modification, which results into a reduced breakdown threshold. The reduction in threshold influences the position of optical breakdown for the succeeding laser pulses and consequently leads to the step-like structures. Additionally, the experimental findings were supplemented with numerical simulations of the influence of reduced damage threshold onto the position of optical breakdown. In summary, chemical material change was defined as cause of the step-like structures. Furthermore, the parameters to avoid these structures were identified.",
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AU - Kopp, Maximilian

AU - Heisterkamp, Alexander

AU - Lubatschowski, Holger

AU - Ripken, Tammo

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