Details
Originalsprache | Englisch |
---|---|
Seiten (von - bis) | 3118-3125 |
Seitenumfang | 8 |
Fachzeitschrift | AIChE journal |
Jahrgang | 52 |
Ausgabenummer | 9 |
Publikationsstatus | Veröffentlicht - 8 Aug. 2006 |
Abstract
The production of O2-enriched air (OEA) using dense mixed conducting perovskite hollow fiber membranes was studied experimentally and theoretically. The fibers were prepared by phase inversion spinning followed by sintering. A mathematical model was developed based on the mass balances for the OEA side, the O2-depleted air side and the hollow fiber itself to simulate the O2-enrichment. Based on the experiments and the model, the mass transport in the mixed conducting material was quantified using Wagner's theory. Furthermore, 3-D plots of broad parameter fields were calculated to estimate optimal operation conditions for a maximum O 2-enrichment. The results elucidate that a required O2 concentration in the OEA, and the production rate can be adjusted by controlling the operation parameters, such as temperature, air pressure differences and sweep airflow rates. The long term operation (800 h) indicates that the perovskite hollow fiber membranes offer a promising potential for the industrial OEA production.
ASJC Scopus Sachgebiete
- Biochemie, Genetik und Molekularbiologie (insg.)
- Biotechnologie
- Umweltwissenschaften (insg.)
- Environmental engineering
- Chemische Verfahrenstechnik (insg.)
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in: AIChE journal, Jahrgang 52, Nr. 9, 08.08.2006, S. 3118-3125.
Publikation: Beitrag in Fachzeitschrift › Artikel › Forschung › Peer-Review
}
TY - JOUR
T1 - Experimental and modeling study of the O2-enrichment by perovskite fibers
AU - Hamel, Christof
AU - Seidel-Morgenstern, Andreas
AU - Schiestel, Thomas
AU - Werth, Steffen
AU - Wang, Haihui
AU - Tablet, Cristina
AU - Caro, Jürgen
PY - 2006/8/8
Y1 - 2006/8/8
N2 - The production of O2-enriched air (OEA) using dense mixed conducting perovskite hollow fiber membranes was studied experimentally and theoretically. The fibers were prepared by phase inversion spinning followed by sintering. A mathematical model was developed based on the mass balances for the OEA side, the O2-depleted air side and the hollow fiber itself to simulate the O2-enrichment. Based on the experiments and the model, the mass transport in the mixed conducting material was quantified using Wagner's theory. Furthermore, 3-D plots of broad parameter fields were calculated to estimate optimal operation conditions for a maximum O 2-enrichment. The results elucidate that a required O2 concentration in the OEA, and the production rate can be adjusted by controlling the operation parameters, such as temperature, air pressure differences and sweep airflow rates. The long term operation (800 h) indicates that the perovskite hollow fiber membranes offer a promising potential for the industrial OEA production.
AB - The production of O2-enriched air (OEA) using dense mixed conducting perovskite hollow fiber membranes was studied experimentally and theoretically. The fibers were prepared by phase inversion spinning followed by sintering. A mathematical model was developed based on the mass balances for the OEA side, the O2-depleted air side and the hollow fiber itself to simulate the O2-enrichment. Based on the experiments and the model, the mass transport in the mixed conducting material was quantified using Wagner's theory. Furthermore, 3-D plots of broad parameter fields were calculated to estimate optimal operation conditions for a maximum O 2-enrichment. The results elucidate that a required O2 concentration in the OEA, and the production rate can be adjusted by controlling the operation parameters, such as temperature, air pressure differences and sweep airflow rates. The long term operation (800 h) indicates that the perovskite hollow fiber membranes offer a promising potential for the industrial OEA production.
KW - Hollow fibers
KW - Mass transfer
KW - Mixed conducting membranes
KW - Oxygen enrichment
KW - Oxygen separation
KW - Perovskite membranes
KW - Reactor modeling
KW - Wagner's theory
UR - http://www.scopus.com/inward/record.url?scp=33748539083&partnerID=8YFLogxK
U2 - 10.1002/aic.10934
DO - 10.1002/aic.10934
M3 - Article
AN - SCOPUS:33748539083
VL - 52
SP - 3118
EP - 3125
JO - AIChE journal
JF - AIChE journal
SN - 0001-1541
IS - 9
ER -