Effect of Recombination Catalyst Loading in PEMWE Membranes on Anodic Hydrogen Content Reduction

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  • Forschungszentrum Jülich
  • Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU Erlangen-Nürnberg)
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Details

OriginalspracheEnglisch
Aufsatznummer124514
FachzeitschriftJournal of the Electrochemical Society
Jahrgang169
Ausgabenummer12
Frühes Online-Datum23 Dez. 2022
PublikationsstatusVeröffentlicht - Dez. 2022

Abstract

Integrating platinum-based recombination catalysts into proton exchange membrane water electrolysis systems effectively reduces the anodic hydrogen content. We studied the effect of the platinum loading of an interlayer close to the anode within the membrane on the anodic hydrogen in oxygen content. For the investigated Pt-loadings between 1 μgPt cm−2 and 140 μgPt cm−2, the results revealed that for a 110 μm membrane, 7 μgPt cm−2 were sufficient to allow a safe operation at cathode pressures up to 10 bar. A further increase of the Pt-loading did not significantly improve the reduction of the anodic hydrogen in oxygen content.

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Ziele für nachhaltige Entwicklung

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Effect of Recombination Catalyst Loading in PEMWE Membranes on Anodic Hydrogen Content Reduction. / Abbas, Dunia; Martin, Agate; Trinke, Patrick et al.
in: Journal of the Electrochemical Society, Jahrgang 169, Nr. 12, 124514, 12.2022.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Abbas D, Martin A, Trinke P, Bierling M, Bensmann B, Thiele S et al. Effect of Recombination Catalyst Loading in PEMWE Membranes on Anodic Hydrogen Content Reduction. Journal of the Electrochemical Society. 2022 Dez;169(12):124514. Epub 2022 Dez 23. doi: 10.1149/1945-7111/aca6a0
Abbas, Dunia ; Martin, Agate ; Trinke, Patrick et al. / Effect of Recombination Catalyst Loading in PEMWE Membranes on Anodic Hydrogen Content Reduction. in: Journal of the Electrochemical Society. 2022 ; Jahrgang 169, Nr. 12.
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abstract = "Integrating platinum-based recombination catalysts into proton exchange membrane water electrolysis systems effectively reduces the anodic hydrogen content. We studied the effect of the platinum loading of an interlayer close to the anode within the membrane on the anodic hydrogen in oxygen content. For the investigated Pt-loadings between 1 μgPt cm−2 and 140 μgPt cm−2, the results revealed that for a 110 μm membrane, 7 μgPt cm−2 were sufficient to allow a safe operation at cathode pressures up to 10 bar. A further increase of the Pt-loading did not significantly improve the reduction of the anodic hydrogen in oxygen content.",
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author = "Dunia Abbas and Agate Martin and Patrick Trinke and Markus Bierling and Boris Bensmann and Simon Thiele and Richard Hanke-Rauschenbach and Thomas B{\"o}hm",
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T1 - Effect of Recombination Catalyst Loading in PEMWE Membranes on Anodic Hydrogen Content Reduction

AU - Abbas, Dunia

AU - Martin, Agate

AU - Trinke, Patrick

AU - Bierling, Markus

AU - Bensmann, Boris

AU - Thiele, Simon

AU - Hanke-Rauschenbach, Richard

AU - Böhm, Thomas

N1 - Funding Information: The authors gratefully acknowledge the financial support from the Federal Ministry of Education and Research of Germany in the framework of PowerMEM (BMBF/03EW0012A).

PY - 2022/12

Y1 - 2022/12

N2 - Integrating platinum-based recombination catalysts into proton exchange membrane water electrolysis systems effectively reduces the anodic hydrogen content. We studied the effect of the platinum loading of an interlayer close to the anode within the membrane on the anodic hydrogen in oxygen content. For the investigated Pt-loadings between 1 μgPt cm−2 and 140 μgPt cm−2, the results revealed that for a 110 μm membrane, 7 μgPt cm−2 were sufficient to allow a safe operation at cathode pressures up to 10 bar. A further increase of the Pt-loading did not significantly improve the reduction of the anodic hydrogen in oxygen content.

AB - Integrating platinum-based recombination catalysts into proton exchange membrane water electrolysis systems effectively reduces the anodic hydrogen content. We studied the effect of the platinum loading of an interlayer close to the anode within the membrane on the anodic hydrogen in oxygen content. For the investigated Pt-loadings between 1 μgPt cm−2 and 140 μgPt cm−2, the results revealed that for a 110 μm membrane, 7 μgPt cm−2 were sufficient to allow a safe operation at cathode pressures up to 10 bar. A further increase of the Pt-loading did not significantly improve the reduction of the anodic hydrogen in oxygen content.

KW - Hydrogen Crossover

KW - Interlayer

KW - PEM Water Electrolysis

KW - Platinum

KW - Recombination

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VL - 169

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