Details
| Originalsprache | Englisch |
|---|---|
| Aufsatznummer | 15651 |
| Fachzeitschrift | Nature Communications |
| Jahrgang | 8 |
| Publikationsstatus | Veröffentlicht - 15 Juni 2017 |
Abstract
Strong-field photoelectron holography and laser-induced electron diffraction (LIED) are two powerful emerging methods for probing the ultrafast dynamics of molecules. However, both of them have remained restricted to static systems and to nuclear dynamics induced by strong-field ionization. Here we extend these promising methods to image purely electronic valence-shell dynamics in molecules using photoelectron holography. In the same experiment, we use LIED and photoelectron holography simultaneously, to observe coupled electronic-rotational dynamics taking place on similar timescales. These results offer perspectives for imaging ultrafast dynamics of molecules on femtosecond to attosecond timescales.
ASJC Scopus Sachgebiete
- Chemie (insg.)
- Allgemeine Chemie
- Biochemie, Genetik und Molekularbiologie (insg.)
- Allgemeine Biochemie, Genetik und Molekularbiologie
- Physik und Astronomie (insg.)
- Allgemeine Physik und Astronomie
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in: Nature Communications, Jahrgang 8, 15651, 15.06.2017.
Publikation: Beitrag in Fachzeitschrift › Artikel › Forschung › Peer-Review
}
TY - JOUR
T1 - Dynamics of valence-shell electrons and nuclei probed by strong-field holography and rescattering
AU - Walt, Samuel G.
AU - Bhargava Ram, Niraghatam
AU - Atala, Marcos
AU - Shvetsov-Shilovskiy, Nikolai Ivanovich
AU - Von Conta, Aaron
AU - Baykusheva, Denitsa
AU - Lein, Manfred
AU - Wörner, Hans Jakob
N1 - Copyright: Copyright 2018 Elsevier B.V., All rights reserved.
PY - 2017/6/15
Y1 - 2017/6/15
N2 - Strong-field photoelectron holography and laser-induced electron diffraction (LIED) are two powerful emerging methods for probing the ultrafast dynamics of molecules. However, both of them have remained restricted to static systems and to nuclear dynamics induced by strong-field ionization. Here we extend these promising methods to image purely electronic valence-shell dynamics in molecules using photoelectron holography. In the same experiment, we use LIED and photoelectron holography simultaneously, to observe coupled electronic-rotational dynamics taking place on similar timescales. These results offer perspectives for imaging ultrafast dynamics of molecules on femtosecond to attosecond timescales.
AB - Strong-field photoelectron holography and laser-induced electron diffraction (LIED) are two powerful emerging methods for probing the ultrafast dynamics of molecules. However, both of them have remained restricted to static systems and to nuclear dynamics induced by strong-field ionization. Here we extend these promising methods to image purely electronic valence-shell dynamics in molecules using photoelectron holography. In the same experiment, we use LIED and photoelectron holography simultaneously, to observe coupled electronic-rotational dynamics taking place on similar timescales. These results offer perspectives for imaging ultrafast dynamics of molecules on femtosecond to attosecond timescales.
UR - http://www.scopus.com/inward/record.url?scp=85020853230&partnerID=8YFLogxK
U2 - 10.1038/ncomms15651
DO - 10.1038/ncomms15651
M3 - Article
C2 - 28643771
AN - SCOPUS:85020853230
VL - 8
JO - Nature Communications
JF - Nature Communications
SN - 2041-1723
M1 - 15651
ER -