Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Autorschaft

  • Sebastian Eckart
  • K. Fehre
  • Nicolas Eicke
  • Andreas Hartung
  • Jonas Rist
  • D. Trabert
  • N. Strenger
  • A. Pier
  • Lothar Ph H. Schmidt
  • Till Jahnke
  • Markus S. Schöffler
  • Manfred Lein
  • Maksim Kunitski
  • Reinhard Dörner

Organisationseinheiten

Externe Organisationen

  • Goethe-Universität Frankfurt am Main
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Details

OriginalspracheEnglisch
Aufsatznummer163202
FachzeitschriftPhysical Review Letters
Jahrgang121
Ausgabenummer16
PublikationsstatusVeröffentlicht - 15 Okt. 2018

Abstract

We report on the nonadiabatic offset of the initial electron momentum distribution in the plane of polarization upon single ionization of argon by strong field tunneling and show how to experimentally control the degree of nonadiabaticity. Two-color counter- and corotating fields (390 and 780 nm) are compared to show that the nonadiabatic offset strongly depends on the temporal evolution of the laser electric field. We introduce a simple method for the direct access to the nonadiabatic offset using two-color counter- and corotating fields. Further, for a single-color circularly polarized field at 780 nm, we show that the radius of the experimentally observed donutlike distribution increases for increasing momentum in the light propagation direction. Our observed initial momentum offsets are well reproduced by the strong-field approximation. A mechanistic picture is introduced that links the measured nonadiabatic offset to the magnetic quantum number of virtually populated intermediate states.

ASJC Scopus Sachgebiete

Zitieren

Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization. / Eckart, Sebastian; Fehre, K.; Eicke, Nicolas et al.
in: Physical Review Letters, Jahrgang 121, Nr. 16, 163202, 15.10.2018.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Eckart, S, Fehre, K, Eicke, N, Hartung, A, Rist, J, Trabert, D, Strenger, N, Pier, A, Schmidt, LPH, Jahnke, T, Schöffler, MS, Lein, M, Kunitski, M & Dörner, R 2018, 'Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization', Physical Review Letters, Jg. 121, Nr. 16, 163202. https://doi.org/10.48550/arXiv.1805.05898, https://doi.org/10.1103/PhysRevLett.121.163202
Eckart, S., Fehre, K., Eicke, N., Hartung, A., Rist, J., Trabert, D., Strenger, N., Pier, A., Schmidt, L. P. H., Jahnke, T., Schöffler, M. S., Lein, M., Kunitski, M., & Dörner, R. (2018). Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization. Physical Review Letters, 121(16), Artikel 163202. https://doi.org/10.48550/arXiv.1805.05898, https://doi.org/10.1103/PhysRevLett.121.163202
Eckart S, Fehre K, Eicke N, Hartung A, Rist J, Trabert D et al. Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization. Physical Review Letters. 2018 Okt 15;121(16):163202. doi: 10.48550/arXiv.1805.05898, 10.1103/PhysRevLett.121.163202
Eckart, Sebastian ; Fehre, K. ; Eicke, Nicolas et al. / Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization. in: Physical Review Letters. 2018 ; Jahrgang 121, Nr. 16.
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title = "Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization",
abstract = "We report on the nonadiabatic offset of the initial electron momentum distribution in the plane of polarization upon single ionization of argon by strong field tunneling and show how to experimentally control the degree of nonadiabaticity. Two-color counter- and corotating fields (390 and 780 nm) are compared to show that the nonadiabatic offset strongly depends on the temporal evolution of the laser electric field. We introduce a simple method for the direct access to the nonadiabatic offset using two-color counter- and corotating fields. Further, for a single-color circularly polarized field at 780 nm, we show that the radius of the experimentally observed donutlike distribution increases for increasing momentum in the light propagation direction. Our observed initial momentum offsets are well reproduced by the strong-field approximation. A mechanistic picture is introduced that links the measured nonadiabatic offset to the magnetic quantum number of virtually populated intermediate states.",
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AU - Rist, Jonas

AU - Trabert, D.

AU - Strenger, N.

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AU - Schmidt, Lothar Ph H.

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AU - Schöffler, Markus S.

AU - Lein, Manfred

AU - Kunitski, Maksim

AU - Dörner, Reinhard

N1 - Funding Information: We thank Yunquan Liu and Armin Scrinzi for helpful discussions. This work was supported by the DFG Priority Programme “Quantum Dynamics in Tailored Intense Fields” of the German Research Foundation (Project No. DO 604/29-1). K. F. and A. H. acknowledge support by the German National Academic Foundation.

PY - 2018/10/15

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