Details
Originalsprache | Englisch |
---|---|
Aufsatznummer | 196801 |
Fachzeitschrift | Physical Review Letters |
Jahrgang | 96 |
Ausgabenummer | 19 |
Publikationsstatus | Veröffentlicht - 16 Mai 2006 |
Abstract
The evolution of the plasmon spectrum of the Si(111) (7×7)-Cs surface has been studied by energy loss spectroscopy individually resolved in energy and momentum during the transition from substrate to Cs overlayer metallization. The multipole plasmon is identified by an extremely narrow angular distribution of the inelastic electron scattering, unaccounted for by standard dipole scattering theory. A crossover between multipole and monopole surface plasmon is observed at finite surface wave vectors q∥, depending on Cs coverage, and reveals a high sensitivity of the short-wavelength multipole components on surface morphology.
ASJC Scopus Sachgebiete
- Physik und Astronomie (insg.)
- Allgemeine Physik und Astronomie
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in: Physical Review Letters, Jahrgang 96, Nr. 19, 196801, 16.05.2006.
Publikation: Beitrag in Fachzeitschrift › Artikel › Forschung › Peer-Review
}
TY - JOUR
T1 - Crossover between monopole and multipole plasmon of Cs monolayers on Si(111) individually resolved in energy and momentum
AU - Zielasek, Volkmar
AU - Rönitz, Neele
AU - Henzler, Martin
AU - Pfnür, Herbert
PY - 2006/5/16
Y1 - 2006/5/16
N2 - The evolution of the plasmon spectrum of the Si(111) (7×7)-Cs surface has been studied by energy loss spectroscopy individually resolved in energy and momentum during the transition from substrate to Cs overlayer metallization. The multipole plasmon is identified by an extremely narrow angular distribution of the inelastic electron scattering, unaccounted for by standard dipole scattering theory. A crossover between multipole and monopole surface plasmon is observed at finite surface wave vectors q∥, depending on Cs coverage, and reveals a high sensitivity of the short-wavelength multipole components on surface morphology.
AB - The evolution of the plasmon spectrum of the Si(111) (7×7)-Cs surface has been studied by energy loss spectroscopy individually resolved in energy and momentum during the transition from substrate to Cs overlayer metallization. The multipole plasmon is identified by an extremely narrow angular distribution of the inelastic electron scattering, unaccounted for by standard dipole scattering theory. A crossover between multipole and monopole surface plasmon is observed at finite surface wave vectors q∥, depending on Cs coverage, and reveals a high sensitivity of the short-wavelength multipole components on surface morphology.
UR - http://www.scopus.com/inward/record.url?scp=33646689061&partnerID=8YFLogxK
U2 - 10.1103/PhysRevLett.96.196801
DO - 10.1103/PhysRevLett.96.196801
M3 - Article
AN - SCOPUS:33646689061
VL - 96
JO - Physical Review Letters
JF - Physical Review Letters
SN - 0031-9007
IS - 19
M1 - 196801
ER -