TY - JOUR

T1 - Correlation of geometrical and electronic properties in metallic nanowires

AU - Pfnür, Herbert

AU - Tegenkamp, Christoph

AU - Czubanowski, M.

AU - Lükermann, Daniel

AU - Rönspies, J. P.

AU - Wießell, S.

PY - 2010/9/7

Y1 - 2010/9/7

N2 - The structure on the atomic scale was found to be directly correlated with the electronic and transport properties of ultra-thin metallic wires. We present examples of both self-organized and artificially structured nanowires in the system Pb/Si(557). We demonstrate that artificial structuring on the nanoscale allows identification and determination of the electrical transport properties of atomic size defects, using Si(557) as a quasi-insulating substrate and a Si double step in a monolayer high Pb nanowire as an example. One-dimensional (1D) properties with strong electron correlation and various instabilities in metallic chains or ribbons generated by metal adsorption of sub-monolayers on insulating substrates like Si(111) or Si(557) turn out to always be modified by the unavoidable coupling to 2D and 3D. The wealth of new and partly unexpected phenomena is exemplified here again in monolayers of Pb on Si(557), which forms wire-like arrays. We identify structural self-stabilization as the origin of 1D electronic transport and show that a new 1D state is generated by step decoration. Magnetoconductance measurements yield even deeper insight into mechanisms of electronic transport, as also exemplified in this specific system.

AB - The structure on the atomic scale was found to be directly correlated with the electronic and transport properties of ultra-thin metallic wires. We present examples of both self-organized and artificially structured nanowires in the system Pb/Si(557). We demonstrate that artificial structuring on the nanoscale allows identification and determination of the electrical transport properties of atomic size defects, using Si(557) as a quasi-insulating substrate and a Si double step in a monolayer high Pb nanowire as an example. One-dimensional (1D) properties with strong electron correlation and various instabilities in metallic chains or ribbons generated by metal adsorption of sub-monolayers on insulating substrates like Si(111) or Si(557) turn out to always be modified by the unavoidable coupling to 2D and 3D. The wealth of new and partly unexpected phenomena is exemplified here again in monolayers of Pb on Si(557), which forms wire-like arrays. We identify structural self-stabilization as the origin of 1D electronic transport and show that a new 1D state is generated by step decoration. Magnetoconductance measurements yield even deeper insight into mechanisms of electronic transport, as also exemplified in this specific system.

KW - Electronic transport

KW - Nanowires

KW - Pb

KW - Si

UR - http://www.scopus.com/inward/record.url?scp=78650490285&partnerID=8YFLogxK

U2 - 10.1002/pssb.201046103

DO - 10.1002/pssb.201046103

M3 - Article

AN - SCOPUS:78650490285

VL - 247

SP - 2509

EP - 2521

JO - Physica Status Solidi (B) Basic Research

JF - Physica Status Solidi (B) Basic Research

SN - 0370-1972

IS - 10

ER -