Characterization of nuclear wave packets describing molecular photodissociation

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  • Julius-Maximilians-Universität Würzburg
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Details

OriginalspracheEnglisch
Seiten (von - bis)3609-3614
Seitenumfang6
FachzeitschriftJournal of Chemical Physics
Jahrgang113
Ausgabenummer9
PublikationsstatusVeröffentlicht - 21 Aug. 2000
Extern publiziertJa

Abstract

This paper shows that it is, in principle, possible to construct complex-valued nuclear wave packets describing photofragments produced through short-pulse excitation. This requires the experimental determination of the fragment kinetic-energy distribution and a pump-probe signal detecting the products. These sets of data yield the wave-packet densities in momentum and coordinate space. The phases of the wave function can be obtained from an iteration scheme. By investigating several examples, this paper shows that the algorithm works excellent even in unfavorable cases.

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Characterization of nuclear wave packets describing molecular photodissociation. / Lein, Manfred; Erdmann, Martin; Engel, Volker.
in: Journal of Chemical Physics, Jahrgang 113, Nr. 9, 21.08.2000, S. 3609-3614.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Lein M, Erdmann M, Engel V. Characterization of nuclear wave packets describing molecular photodissociation. Journal of Chemical Physics. 2000 Aug 21;113(9):3609-3614. doi: 10.1063/1.1287718
Lein, Manfred ; Erdmann, Martin ; Engel, Volker. / Characterization of nuclear wave packets describing molecular photodissociation. in: Journal of Chemical Physics. 2000 ; Jahrgang 113, Nr. 9. S. 3609-3614.
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