Absorption and multi-phonon quenching in nanocrystal doped SiO2 fibers

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OriginalspracheEnglisch
Seiten (von - bis)1631-1642
Seitenumfang12
FachzeitschriftOptical materials express
Jahrgang11
Ausgabenummer6
Frühes Online-Datum6 Mai 2021
PublikationsstatusVeröffentlicht - Juni 2021

Abstract

SiO 2 fibers doped with rare-earth-doped nanocrystals are promising to overcome the strong SiO 2 multi-phonon quenching and could yield novel laser gain materials. So far, no attention has been paid to the question how well the nanocrystals can suppress the quenching depending on the properties of the SiO 2 host glass. Here, a novel analytical model was applied to study the impact of the glass purity and composition on the quenching efficiency. Only a few experimentally accessible material and design parameters are required to compute the average quenching rate inside the nanocrystals. It is demonstrated that sufficiently low levels of quenching can only be expected for SiO 2 free of impurities or dopants that increase the multi-phonon absorption. This indicates that high-purity aluminosilicate glasses, in contrast to phosphosilicate and borosilicate glasses, are ideal hosts.

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Absorption and multi-phonon quenching in nanocrystal doped SiO2 fibers. / Steinke, Michael; Spelthann, Simon; Rühl, Axel et al.
in: Optical materials express, Jahrgang 11, Nr. 6, 06.2021, S. 1631-1642.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Steinke, M, Spelthann, S, Rühl, A & Ristau, D 2021, 'Absorption and multi-phonon quenching in nanocrystal doped SiO2 fibers', Optical materials express, Jg. 11, Nr. 6, S. 1631-1642. https://doi.org/10.1364/OME.424116
Steinke M, Spelthann S, Rühl A, Ristau D. Absorption and multi-phonon quenching in nanocrystal doped SiO2 fibers. Optical materials express. 2021 Jun;11(6):1631-1642. Epub 2021 Mai 6. doi: 10.1364/OME.424116
Steinke, Michael ; Spelthann, Simon ; Rühl, Axel et al. / Absorption and multi-phonon quenching in nanocrystal doped SiO2 fibers. in: Optical materials express. 2021 ; Jahrgang 11, Nr. 6. S. 1631-1642.
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abstract = "SiO 2 fibers doped with rare-earth-doped nanocrystals are promising to overcome the strong SiO 2 multi-phonon quenching and could yield novel laser gain materials. So far, no attention has been paid to the question how well the nanocrystals can suppress the quenching depending on the properties of the SiO 2 host glass. Here, a novel analytical model was applied to study the impact of the glass purity and composition on the quenching efficiency. Only a few experimentally accessible material and design parameters are required to compute the average quenching rate inside the nanocrystals. It is demonstrated that sufficiently low levels of quenching can only be expected for SiO 2 free of impurities or dopants that increase the multi-phonon absorption. This indicates that high-purity aluminosilicate glasses, in contrast to phosphosilicate and borosilicate glasses, are ideal hosts. ",
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note = "Funding Information: Funding. Deutsche Forschungsgemeinschaft (Cluster of Excellence PhoenixD (EXC 2122), EXC-2123 Quantum Frontiers - 390837967); European Social Fund (EFRE-SER 2014-2020, 85003655, 85003502); Nieders{\"a}chsisches Ministerium f{\"u}r Wissenschaft und Kultur (“Quanten-und Nanometrologie” (QUANOMET)). ",
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AU - Steinke, Michael

AU - Spelthann, Simon

AU - Rühl, Axel

AU - Ristau, Detlev

N1 - Funding Information: Funding. Deutsche Forschungsgemeinschaft (Cluster of Excellence PhoenixD (EXC 2122), EXC-2123 Quantum Frontiers - 390837967); European Social Fund (EFRE-SER 2014-2020, 85003655, 85003502); Niedersächsisches Ministerium für Wissenschaft und Kultur (“Quanten-und Nanometrologie” (QUANOMET)).

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AB - SiO 2 fibers doped with rare-earth-doped nanocrystals are promising to overcome the strong SiO 2 multi-phonon quenching and could yield novel laser gain materials. So far, no attention has been paid to the question how well the nanocrystals can suppress the quenching depending on the properties of the SiO 2 host glass. Here, a novel analytical model was applied to study the impact of the glass purity and composition on the quenching efficiency. Only a few experimentally accessible material and design parameters are required to compute the average quenching rate inside the nanocrystals. It is demonstrated that sufficiently low levels of quenching can only be expected for SiO 2 free of impurities or dopants that increase the multi-phonon absorption. This indicates that high-purity aluminosilicate glasses, in contrast to phosphosilicate and borosilicate glasses, are ideal hosts.

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