A new resonant Laser-SNMS system for environmental ultra-trace analysis: Installation and optimization

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Autoren

  • Michael Franzmann
  • Hauke Bosco
  • Clemens Walther
  • Klaus Wendt

Externe Organisationen

  • Johannes Gutenberg-Universität Mainz
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Details

OriginalspracheEnglisch
Seiten (von - bis)27-32
Seitenumfang6
FachzeitschriftInternational Journal of Mass Spectrometry
Jahrgang423
PublikationsstatusVeröffentlicht - 10 Okt. 2017

Abstract

Localization, analysis and mobility of radioactive contaminated particles is of major concern for assessment of contamination threads and nuclear forensics. For this purpose, a new resonant Laser-SNMS system was developed and set up at the Institute for Radioecology and Radiation Protection for spatially resolved ultra-trace analysis of low concentrated radionuclides directly on environmental samples. This paper describes the adaption and combination of a dedicated Ti:sapphire laser system with a commercial TOF-SIMS instrument for resonant Laser-SNMS. The project includes computer simulations for optimization of the TOF analyzer. Results on synthetic uranium and technetium samples verify the expected excellent suppression of interfering isobaric contaminations.

ASJC Scopus Sachgebiete

Zitieren

A new resonant Laser-SNMS system for environmental ultra-trace analysis: Installation and optimization. / Franzmann, Michael; Bosco, Hauke; Walther, Clemens et al.
in: International Journal of Mass Spectrometry, Jahrgang 423, 10.10.2017, S. 27-32.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Franzmann M, Bosco H, Walther C, Wendt K. A new resonant Laser-SNMS system for environmental ultra-trace analysis: Installation and optimization. International Journal of Mass Spectrometry. 2017 Okt 10;423:27-32. doi: 10.1016/j.ijms.2017.10.003
Franzmann, Michael ; Bosco, Hauke ; Walther, Clemens et al. / A new resonant Laser-SNMS system for environmental ultra-trace analysis : Installation and optimization. in: International Journal of Mass Spectrometry. 2017 ; Jahrgang 423. S. 27-32.
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abstract = "Localization, analysis and mobility of radioactive contaminated particles is of major concern for assessment of contamination threads and nuclear forensics. For this purpose, a new resonant Laser-SNMS system was developed and set up at the Institute for Radioecology and Radiation Protection for spatially resolved ultra-trace analysis of low concentrated radionuclides directly on environmental samples. This paper describes the adaption and combination of a dedicated Ti:sapphire laser system with a commercial TOF-SIMS instrument for resonant Laser-SNMS. The project includes computer simulations for optimization of the TOF analyzer. Results on synthetic uranium and technetium samples verify the expected excellent suppression of interfering isobaric contaminations.",
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AU - Franzmann, Michael

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AU - Walther, Clemens

AU - Wendt, Klaus

N1 - Funding information: This research has been financially supported by the German Federal Ministry of Education and Research (BMBF) in the joint project SIRIUS. We also thank S. Kayser and W. Paul from the company IONTOF for their support during assembly and simulation based optimization of the Laser-SNMS system. Additional, M. Franzmann thanks the Siebold-Sasse Foundation for financial support.

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